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室温下钙钛矿超表面中80%激子分数极化激元的远程弹道传播

Long-Range Ballistic Propagation of 80% Excitonic Fraction Polaritons in a Perovskite Metasurface at Room Temperature.

作者信息

Dang Nguyen Ha My, Zanotti Simone, Drouard Emmanuel, Chevalier Céline, Trippé-Allard Gaëlle, Deleporte Emmanuelle, Seassal Christian, Gerace Dario, Nguyen Hai Son

机构信息

Université Lyon, Ecole Centrale de Lyon, CNRS, INSA Lyon, Université Claude Bernard Lyon 1, CPE Lyon, CNRS, INL, UMR5270, Ecully 69130, France.

Dipartimento di Fisica, Università di Pavia, via Bassi 6, I-27100 Pavia, Italy.

出版信息

Nano Lett. 2024 Sep 25;24(38):11839-11846. doi: 10.1021/acs.nanolett.4c02696. Epub 2024 Sep 13.

Abstract

Exciton-polaritons, hybrid light-matter excitations arising from the strong coupling between excitons in semiconductors and photons in photonic nanostructures, are crucial for exploring the physics of quantum fluids of light and developing all-optical devices. Achieving room temperature propagation of polaritons with a large excitonic fraction is challenging but vital, e.g., for nonlinear light transport. We report on room temperature propagation of exciton-polaritons in a metasurface made from a subwavelength lattice of perovskite pillars. The large Rabi splitting, much greater than the optical phonon energy, decouples the lower polariton band from the phonon bath of the perovskite. These cooled polaritons, in combination with the high group velocity achieved through the metasurface design, enable long-range propagation, exceeding hundreds of micrometers even with an 80% excitonic component. Furthermore, the design of the metasurface introduces an original mechanism for unidirectional propagation through polarization control, suggesting a new avenue for the development of advanced polaritonic devices.

摘要

激子极化激元是半导体中的激子与光子纳米结构中的光子之间强耦合产生的混合光物质激发态,对于探索光量子流体的物理性质和开发全光器件至关重要。实现具有大激子分数的极化激元在室温下的传播具有挑战性,但却至关重要,例如对于非线性光传输而言。我们报道了激子极化激元在由钙钛矿柱亚波长晶格构成的超表面中的室温传播情况。大的拉比分裂远大于光学声子能量,使较低的极化激元能带与钙钛矿的声子库解耦。这些冷却的极化激元,再加上通过超表面设计实现的高群速度,能够实现长距离传播,即使激子成分占80%,传播距离也能超过数百微米。此外,超表面的设计引入了一种通过偏振控制实现单向传播的独特机制,为先进极化激元器件的开发开辟了一条新途径。

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