Wang Nan, Li Jianbo, Wang Chong, Zhang Xiaoqi, Ding Song, Guo Zexuan, Duan Yuhan, Jiang Dayong
School of Engineering, Changchun Normal University, Changchun 130032, China.
Engineering Research Center of Jilin Province Rare Metal Deep Processing, Changchun 130022, China.
Nanomaterials (Basel). 2024 Sep 4;14(17):1442. doi: 10.3390/nano14171442.
Ultraviolet (UV) photodetectors (PDs) based on nanowire (NW) hold significant promise for applications in fire detection, optical communication, and environmental monitoring. As optoelectronic devices evolve towards lower dimensionality, multifunctionality, and integrability, multicolor PDs have become a research hotspot in optics and electronic information. This study investigates the enhancement of detection capability in a light-trapping ZnO NW array through modification with Pt nanoparticles (NPs) via magnetron sputtering and hydrothermal synthesis. The optimized PD exhibits superior performance, achieving a responsivity of 12.49 A/W, detectivity of 4.07 × 10 Jones, and external quantum efficiency (EQE) of 4.19 × 10%, respectively. In addition, the Pt NPs/ZnO NW/ZnO PD maintains spectral selectivity in the UV region. These findings show the pivotal role of Pt NPs in enhancing photodetection performance through their strong light absorption and scattering properties. This improvement is associated with localized surface plasmon resonance induced by the Pt NPs, leading to enhanced incident light and interfacial charge separation for the specialized configurations of the nanodevice. Utilizing metal NPs for device modification represents a breakthrough that positively affects the preparation of high-performance ZnO-based UV PDs.
基于纳米线(NW)的紫外(UV)光电探测器(PDs)在火灾探测、光通信和环境监测等应用中具有巨大的潜力。随着光电器件朝着更低维度、多功能性和可集成性发展,多色光电探测器已成为光学和电子信息领域的研究热点。本研究通过磁控溅射和水热合成法用铂纳米颗粒(NPs)对光捕获ZnO纳米线阵列进行改性,研究其探测能力的增强。优化后的光电探测器表现出优异的性能,响应度分别达到12.49 A/W、探测率达到4.07×10 Jones以及外量子效率(EQE)达到4.19×10%。此外,Pt NPs/ZnO NW/ZnO光电探测器在紫外区域保持光谱选择性。这些发现表明Pt NPs通过其强光吸收和散射特性在提高光电探测性能方面起着关键作用。这种改进与Pt NPs诱导的局域表面等离子体共振有关,导致纳米器件特殊结构的入射光增强和界面电荷分离。利用金属纳米颗粒对器件进行改性是一项突破,对高性能ZnO基紫外光电探测器的制备产生了积极影响。