Gu Minghui, Sheng Haohao, Wu Xiaofeng, Wu Mei, Liu Xiaoran, Yang Fang, Zhang Zhongshan, Gao Peng, Wang Zhijun, Meng Meng, Guo Jiandong
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100190, China.
Natl Sci Rev. 2023 Nov 21;11(10):nwad296. doi: 10.1093/nsr/nwad296. eCollection 2024 Oct.
Spin texture in -space is a consequence of spin splitting due to strong spin-orbit coupling and inversion symmetry breaking. It underlies fertile spin transport phenomena and is of crucial importance for spintronics. Here, we observe the spin texture in -space of nominally centrosymmetric SrIrO grown on NdGaO (110) substrates, using non-linear magnetotransport measurements. We demonstrate that the spin texture is not only induced by the interface, which inherently breaks the inversion symmetry in strong spin-orbit coupled SrIrO films, but also originates from the film bulk. Structural analysis reveals that thicker SrIrO films exhibit a strain gradient, which could be considered as a continuous change in the lattice constant across different layers and breaks the inversion symmetry throughout the entire SrIrO films, giving rise to the spin texture in -space. First-principles calculations reveal that the strain gradient creates large spin-splitting bands, inducing the spin texture with anisotropy, which is consistent with our experimental observations. Our results offer an efficient method for inducing the spin textures in -space.
空间中的自旋纹理是由于强自旋轨道耦合和反演对称性破缺导致的自旋分裂的结果。它是丰富的自旋输运现象的基础,对自旋电子学至关重要。在这里,我们使用非线性磁输运测量方法,观察了在NdGaO(110)衬底上生长的名义上中心对称的SrIrO的空间自旋纹理。我们证明,自旋纹理不仅由界面诱导,界面在强自旋轨道耦合的SrIrO薄膜中固有地打破了反演对称性,而且还起源于薄膜本体。结构分析表明,较厚的SrIrO薄膜表现出应变梯度,这可以被认为是晶格常数在不同层之间的连续变化,并在整个SrIrO薄膜中打破了反演对称性,从而产生了空间中的自旋纹理。第一性原理计算表明,应变梯度产生了大的自旋分裂带,诱导了具有各向异性的自旋纹理,这与我们的实验观察结果一致。我们的结果提供了一种在空间中诱导自旋纹理的有效方法。