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磁性 Kagome 拓扑金属 FeSn 薄膜中高电子迁移率的证据。

Evidence of high electron mobility in magnetic kagome topological metal FeSn thin films.

作者信息

Mosesso Lorenzo, Tomarchio Luca, Bhattarai Niraj, Macis Salvatore, Gori Paola, Grilli Antonio, Cestelli Guidi Mariangela, Philip John, Pulci Olivia, Lupi Stefano

机构信息

Department of Physics, Sapienza University Piazzale Aldo Moro 5 00185 Rome Italy

INFN Section of Rome P. Le Aldo Moro, 2 00185 Rome Italy.

出版信息

Nanoscale Adv. 2024 Oct 14;6(24):6378-85. doi: 10.1039/d4na00737a.

Abstract

We present a systematic study of the low-energy electrodynamics of the magnetic FeSn kagome metal, which hosts both topological (Dirac) and non-trivial states. Our results reveal that the optical conductivity of FeSn shows two Drude contributions that can be associated with the linear (Dirac) and parabolic (massive) bands, with a dominance of the former to the DC conductivity at low temperatures. The weight of the Drude response shifts toward lower frequencies upon cooling due to a rapid increase in the Dirac electron mobility, which we associate with a temperature suppression of e-ph scattering. The experimental interband dielectric function is in very good agreement with that calculated within Density Functional Theory (DFT). These results provide a full description of the charge dynamics in FeSn kagome topological metal, opening the road for its use in photonic and plasmonic applications.

摘要

我们对磁性FeSn Kagome金属的低能电动力学进行了系统研究,该金属同时具有拓扑(狄拉克)态和非平凡态。我们的结果表明,FeSn的光导率显示出两个德鲁德贡献,可分别与线性(狄拉克)带和抛物线(有质量)带相关联,在低温下前者对直流电导率起主导作用。由于狄拉克电子迁移率的快速增加,德鲁德响应的权重在冷却时向低频移动,我们将其与电子-声子散射的温度抑制相关联。实验得到的带间介电函数与密度泛函理论(DFT)计算的结果非常吻合。这些结果全面描述了FeSn Kagome拓扑金属中的电荷动力学,为其在光子和等离子体应用中的使用开辟了道路。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/89dc/11614061/85a224a2dc46/d4na00737a-f1.jpg

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