Key Laboratory of Chemical Utilization of Plant Resources of Nanchang, Institute of Functional Materials and Agricultural Applied Chemistry, College of Chemistry and Material, Jiangxi Agricultural University, Nanchang, 330045, PR China.
School of Resources and Environment, University of Electronic Science and Technology of China, Chengdu, 611731, PR China.
Mikrochim Acta. 2024 Nov 29;191(12):771. doi: 10.1007/s00604-024-06828-w.
The introduction of comprehensive health, related to human living environment and mental state, helps people to improve human health literacy and accept scientific health guidance. The unique structure and properties of black phosphorene (BP) provide potential opportunities for rapid development and versatile applications of high-performance sensors serving comprehensive health. The review begins with the preparation from bulk black phosphorous crystals via transforming requirements of phosphorous allotropes and BP nanosheets via preparative strategies using both "top-down" and "bottom-up" methods. Then the diversified modification of BP and versatile fabrication of diversified bio-/chemo-nanosensors for sensitive detection of analytes are discussed. Besides, the challenges including the preparation of BP, diversified modification, devices for improving performance defects and chemo-/bio-nanosensors for enhancing performance are outlined together with potential opportunities for the BP preparation and applications in comprehensive health from agricultural environments, food safety, personal life, physical and mental life, and finally to medical care.
综合健康的引入，与人类生活环境和精神状态有关，有助于提高人类健康素养，接受科学健康指导。黑磷烯（BP）独特的结构和性质为高性能传感器的快速发展和多功能应用提供了潜在的机会，这些传感器服务于综合健康。本综述首先从块状黑磷晶体的制备开始，通过转变磷同素异形体和 BP 纳米片的要求，采用“自上而下”和“自下而上”的方法制备策略。然后讨论了 BP 的多样化修饰和多功能生物/化学纳米传感器的广泛制备，用于灵敏检测分析物。此外，还概述了包括 BP 的制备、多样化修饰、器件性能缺陷改善和化学/生物纳米传感器性能增强在内的挑战，以及从农业环境、食品安全、个人生活、身心健康到医疗保健等方面，BP 制备和应用于综合健康的潜在机遇。
