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半金属TaSb的拓扑表面态

Topological surface states of semimetal TaSb.

作者信息

Lee Ji-Eun, Liu Yu, Hwang Jinwoong, Hwang Choongyu, Petrovic Cedomir, Park Se Young, Ryu Hyejin, Mo Sung-Kwan

机构信息

Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

Center for Spintronics, Korea Institute of Science and Technology (KIST), Seoul, 02792, South Korea.

出版信息

Nano Converg. 2024 Dec 2;11(1):50. doi: 10.1186/s40580-024-00457-y.

DOI:10.1186/s40580-024-00457-y
PMID:39621287
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11612110/
Abstract

Topological surface states, protected by the global symmetry of the materials, are the keys to understanding various novel electrical, magnetic, and optical properties. TaSb is a newly discovered topological material with unique transport phenomena, including negative magnetoresistance and resistivity plateau, whose microscopic understanding is yet to be reached. In this study, we investigate the electronic band structure of TaSb using angle-resolved photoemission spectroscopy and density functional theory. Our analyses reveal distinct bulk and surface states in TaSb, providing direct evidence of its topological nature. Notably, surface states predominate the electronic contribution near the Fermi level, while bulk bands are mostly located at higher binding energies. Our study underlines the importance of systematic investigations into the electronic structures of topological materials, offering insights into their fundamental properties and potential applications in future technologies.

摘要

由材料的全局对称性保护的拓扑表面态是理解各种新颖电学、磁学和光学性质的关键。TaSb是一种新发现的具有独特输运现象的拓扑材料,包括负磁阻和电阻率平台,其微观理解尚未达成。在本研究中,我们使用角分辨光电子能谱和密度泛函理论研究了TaSb的电子能带结构。我们的分析揭示了TaSb中明显的体态和表面态,为其拓扑性质提供了直接证据。值得注意的是,表面态在费米能级附近的电子贡献中占主导地位,而体态大多位于更高的结合能处。我们的研究强调了对拓扑材料电子结构进行系统研究的重要性,为其基本性质和未来技术中的潜在应用提供了见解。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4487/11612110/2339b6c91261/40580_2024_457_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4487/11612110/2c03afc9c913/40580_2024_457_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4487/11612110/aa31d34bbe98/40580_2024_457_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4487/11612110/a09b9e5b998d/40580_2024_457_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4487/11612110/2339b6c91261/40580_2024_457_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4487/11612110/2c03afc9c913/40580_2024_457_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4487/11612110/aa31d34bbe98/40580_2024_457_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4487/11612110/a09b9e5b998d/40580_2024_457_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4487/11612110/2339b6c91261/40580_2024_457_Fig4_HTML.jpg

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本文引用的文献

1
Nanoscale inhomogeneity and the evolution of correlation strength in FeSeS.FeSeS中的纳米级不均匀性与关联强度的演变
Nano Converg. 2023 Dec 22;10(1):59. doi: 10.1186/s40580-023-00405-2.
2
Recent progress of exciton transport in two-dimensional semiconductors.二维半导体中激子输运的最新进展。
Nano Converg. 2023 Dec 15;10(1):57. doi: 10.1186/s40580-023-00404-3.
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Electronic structure in a transition metal dipnictide TaAs.
J Phys Condens Matter. 2023 Nov 14;36(7). doi: 10.1088/1361-648X/ad04fc.
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Topological quantum devices: a review.拓扑量子器件:综述
Nanoscale. 2023 Aug 10;15(31):12787-12817. doi: 10.1039/d3nr01288c.
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Enhanced thermoelectric performance of SnSe by controlled vacancy population.通过控制空位数量提高SnSe的热电性能。
Nano Converg. 2023 Jul 7;10(1):32. doi: 10.1186/s40580-023-00381-7.
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Anisotropy of impact ionization in WSe field effect transistors.WSe 场效应晶体管中碰撞电离的各向异性
Nano Converg. 2023 Mar 17;10(1):13. doi: 10.1186/s40580-023-00361-x.
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Investigation of the mechanism of the anomalous Hall effects in CrTe/(BiSb)(TeSe) heterostructure.CrTe/(BiSb)(TeSe)异质结构中反常霍尔效应机制的研究。
Nano Converg. 2023 Jan 10;10(1):2. doi: 10.1186/s40580-022-00348-0.
8
Two-Dimensional Van Der Waals Topological Materials: Preparation, Properties, and Device Applications.二维范德华拓扑材料:制备、性质及器件应用
Small. 2022 Nov;18(47):e2204380. doi: 10.1002/smll.202204380. Epub 2022 Sep 22.
9
2D materials: increscent quantum flatland with immense potential for applications.二维材料:具有巨大应用潜力的新兴量子平面
Nano Converg. 2022 Jun 6;9(1):26. doi: 10.1186/s40580-022-00317-7.
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Criteria for Realizing Room-Temperature Electrical Transport Applications of Topological Materials.
Adv Mater. 2020 Dec;32(50):e2005698. doi: 10.1002/adma.202005698. Epub 2020 Nov 3.