Parfenov Oleg E, Averyanov Dmitry V, Sokolov Ivan S, Mihalyuk Alexey N, Kondratev Oleg A, Taldenkov Alexander N, Tokmachev Andrey M, Storchak Vyacheslav G
National Research Center "Kurchatov Institute", Kurchatov Sq. 1, Moscow, 123182, Russia.
Institute of High Technologies and Advanced Materials, Far Eastern Federal University, Vladivostok, 690950, Russia.
Adv Mater. 2025 Jan;37(4):e2412321. doi: 10.1002/adma.202412321. Epub 2024 Dec 8.
2D magnets have emerged as a class of materials highly promising for studies of quantum phenomena and applications in ultra-compact spintronics. Current research aims at design of 2D magnets with particular functional properties. A formidable challenge is to produce metallic monolayers: the material landscape of layered magnetic systems is strongly dominated by insulators; rare metallic magnets, such as FeGeTe, become insulating as they approach the monolayer limit. Here, electron transport measurements demonstrate that the recently discovered 2D magnet GdAlSi - graphene-like AlSi layers coupled to layers of Gd atoms - remains metallic down to a single monolayer. Band structure analysis indicates the material to be an electride, which may stabilize the metallic state. Remarkably, the sheet conductance of 2D GdAlSi is proportional to the number of monolayers - a manifestation of scalable conductivity. The GdAlSi layers are epitaxially integrated with silicon, facilitating applications in electronics.
二维磁体已成为一类在量子现象研究和超紧凑型自旋电子学应用中极具前景的材料。当前的研究旨在设计具有特定功能特性的二维磁体。一个巨大的挑战是制备金属单层:层状磁系统的材料格局在很大程度上由绝缘体主导;像FeGeTe这样稀有的金属磁体在接近单层极限时会变成绝缘体。在此,电子输运测量表明,最近发现的二维磁体GdAlSi(类似于石墨烯的AlSi层与Gd原子层耦合)即使在单层时仍保持金属性。能带结构分析表明该材料是一种电子化合物,这可能使金属态得以稳定。值得注意的是,二维GdAlSi的面电导与单层数量成正比——这是可扩展导电性的一种表现。GdAlSi层与硅外延集成,便于在电子学中的应用。