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砷化钙中接近莫特-约菲-雷格尔极限处的量子振荡观测。

Observation of quantum oscillations near the Mott-Ioffe-Regel limit in CaAs.

作者信息

Wang Yuxiang, Zhao Minhao, Zhang Jinglei, Wu Wenbin, Li Shichao, Zhang Yong, Jiang Wenxiang, Joseph Nesta Benno, Xu Liangcai, Mou Yicheng, Yang Yunkun, Leng Pengliang, Zhang Yong, Pi Li, Suslov Alexey, Ozerov Mykhaylo, Wyzula Jan, Orlita Milan, Zhu Fengfeng, Zhang Yi, Kou Xufeng, Zhu Zengwei, Narayan Awadhesh, Qian Dong, Wen Jinsheng, Yuan Xiang, Xiu Faxian, Zhang Cheng

机构信息

State Key Laboratory of Surface Physics and Institute for Nanoelectronic Devices and Quantum Computing, Fudan University, Shanghai 200433, China.

State Key Laboratory of Surface Physics and Department of Physics, Fudan University, Shanghai 200433, China.

出版信息

Natl Sci Rev. 2024 Mar 29;11(12):nwae127. doi: 10.1093/nsr/nwae127. eCollection 2024 Dec.

Abstract

The Mott-Ioffe-Regel limit sets the lower bound of the carrier mean free path for coherent quasiparticle transport. Metallicity beyond this limit is of great interest because it is often closely related to quantum criticality and unconventional superconductivity. Progress along this direction mainly focuses on the strange-metal behaviors originating from the evolution of the quasiparticle scattering rate, such as linear-in-temperature resistivity, while the quasiparticle coherence phenomena in this regime are much less explored due to the short mean free path at the diffusive bound. Here we report the observation of quantum oscillations from Landau quantization near the Mott-Ioffe-Regel limit in CaAs. Despite the insulator-like temperature dependence of resistivity, CaAs presents giant magnetoresistance and prominent Shubnikov-de Haas oscillations from Fermi surfaces, indicating highly coherent band transport. In contrast, quantum oscillation is absent in the magnetic torque. The quasiparticle effective mass increases systematically with magnetic fields, manifesting a much larger value than what is expected based on magneto-infrared spectroscopy. This suggests a strong many-body renormalization effect near the Fermi surface. We find that these unconventional behaviors may be explained by the interplay between the mobility edge and the van Hove singularity, which results in the formation of coherent cyclotron orbits emerging at the diffusive bound. Our results call for further study on the electron correlation effect of the van Hove singularity.

摘要

莫特-约费-雷格尔极限设定了相干准粒子输运中载流子平均自由程的下限。超出此极限的金属性备受关注,因为它通常与量子临界性和非常规超导密切相关。沿此方向的进展主要集中在源于准粒子散射率演化的奇异金属行为上,例如线性温度电阻率,而由于扩散边界处平均自由程较短,该区域的准粒子相干现象研究较少。在此,我们报告了在CaAs中接近莫特-约费-雷格尔极限处从朗道量子化观测到的量子振荡。尽管电阻率具有类似绝缘体的温度依赖性,但CaAs呈现出巨大的磁电阻以及来自费米面的显著舒布尼科夫-德哈斯振荡,表明存在高度相干的能带输运。相比之下,磁转矩中不存在量子振荡。准粒子有效质量随磁场系统性增加,其值比基于磁红外光谱预期的要大得多。这表明在费米面附近存在强烈的多体重整化效应。我们发现,这些非常规行为可能由迁移率边和范霍夫奇点之间的相互作用来解释,这导致在扩散边界处形成相干回旋轨道。我们的结果呼吁进一步研究范霍夫奇点的电子关联效应。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e3a7/11660949/336a35ab2924/nwae127fig1.jpg

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