Bae Junghyun, Yoon Jinsik, Oh Sangmin, Kim Kibeom, Kim Hyeli, Hur Kahyun, Cho Hyesung, Park Wook
Department of Electronics and Information Convergence Engineering, Kyung Hee University, Yongin-si, Republic of Korea.
Extreme Materials Research Center, Advanced Materials Research Division, Korea Institute of Science and Technology, Seoul, Republic of Korea.
Nat Commun. 2024 Dec 30;15(1):10794. doi: 10.1038/s41467-024-54976-7.
Self-assembled configurations are versatile for applications in which liquid-mediated phenomena are employed to ensure that static or mild physical interactions between assembling blocks take advantage of local energy minima. For granular materials, however, a particle's momentum in air leads to random collisions and the formation of disordered phases, eventually producing jammed configurations when densely packed. Therefore, unlike fluidic self-assembly, the self-assembly of dry particles typically lacks programmability based on density and ordering symmetry and has thus been limited in applications. Here, we present the self-assembly of particles with momentum, yielding regular arrays with programmable density and symmetry. The key is to embed anti-repellent structures, i.e. traps, that can capture kinetic particles individually and then robustly hold them against collisions with other momentum granules during a dynamic assembly procedure. By using anti-repellent traps, physical interactions between neighbouring particles can be inhibited, resolving many phenomena related to the uncertainty of space-sharing events in granular packing. With our self-assembly strategy, highly dense yet unjammed configurations are demonstrated, which conserve the inherent randomness in the location information of each granule in the trap and are useful for robust multilevel authentication systems as unique applications.
自组装构型在利用液体介导现象以确保组装单元之间的静态或温和物理相互作用利用局部能量极小值的应用中具有通用性。然而,对于颗粒材料,颗粒在空气中的动量会导致随机碰撞和无序相的形成,当密集堆积时最终会产生堵塞构型。因此,与流体自组装不同,干颗粒的自组装通常缺乏基于密度和有序对称性的可编程性,因此在应用中受到限制。在此,我们展示了具有动量的颗粒的自组装,产生具有可编程密度和对称性的规则阵列。关键在于嵌入抗排斥结构,即陷阱,其能够在动态组装过程中单独捕获运动颗粒,然后牢固地保持它们以防止与其他具有动量的颗粒碰撞。通过使用抗排斥陷阱,可以抑制相邻颗粒之间的物理相互作用,解决许多与颗粒堆积中空间共享事件的不确定性相关的现象。通过我们的自组装策略,展示了高密度但未堵塞的构型,其保留了陷阱中每个颗粒位置信息的固有随机性,并且作为独特应用对于强大的多级认证系统很有用。