Recent Advances in Two-Dimensional Ferromagnetic Materials-Based van der Waals Heterostructures.

Two-dimensional (2D) ferromagnetic materials are subjects of intense research owing to their intriguing physicochemical properties, which hold great potential for fundamental research and spintronic applications. Specifically, 2D van der Waals (vdW) ferromagnetic materials retain both structural integrity and chemical stability even at the monolayer level. Moreover, due to their atomic thickness, these materials can be easily manipulated by stacking them with other 2D vdW ferroic and nonferroic materials, enabling precise control over their physical properties and expanding their functional applications. Consequently, 2D vdW ferromagnetic materials-based heterostructures offer a platform to tailor magnetic properties and explore advanced spintronic devices. This review aims to provide an overview of recent developments in emerging 2D vdW ferromagnetic materials-based heterostructures and devices. The fabrication approaches for 2D ferromagnetic vdW heterostructures are primarily summarized, followed by a review of two categories of heterostructures: ferromagnetic/ferroic and ferromagnetic/nonferroic vdW heterostructures. Subsequently, the progress made in modulating magnetic properties and emergence of various phenomena in these heterostructures is highlighted. Furthermore, the applications of such heterostructures in spintronic devices are discussed along with their future perspectives and potential directions in this exciting field.