Accelerating Plasmonic Hydrogen Sensors for Inert Gas Environments by Transformer-Based Deep Learning.

Rapidly detecting hydrogen leaks is critical for the safe large-scale implementation of hydrogen technologies. However, to date, no technically viable sensor solution exists that meets the corresponding response time targets under technically relevant conditions. Here, we demonstrate how a tailored long short-term transformer ensemble model for accelerated sensing (LEMAS) speeds up the response of an optical plasmonic hydrogen sensor by up to a factor of 40 and eliminates its intrinsic pressure dependence in an environment emulating the inert gas encapsulation of large-scale hydrogen installations by accurately predicting its response value to a hydrogen concentration change before it is physically reached by the sensor hardware. Moreover, LEMAS provides a measure for the uncertainty of the predictions that are pivotal for safety-critical sensor applications. Our results advertise the use of deep learning for the acceleration of sensor response, also beyond the realm of plasmonic hydrogen detection.