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压缩电子背散射衍射成像

Compressive electron backscatter diffraction imaging.

作者信息

Broad Zoë, Robinson Alex W, Wells Jack, Nicholls Daniel, Moshtaghpour Amirafshar, Kirkland Angus I, Browning Nigel D

机构信息

Department of Mechanical, Materials and Aerospace Engineering, University of Liverpool, Liverpool, UK.

SenseAI Innovations Ltd., Liverpool, UK.

出版信息

J Microsc. 2025 Apr;298(1):44-57. doi: 10.1111/jmi.13379. Epub 2025 Jan 11.

DOI:10.1111/jmi.13379
PMID:39797608
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11891967/
Abstract

Electron backscatter diffraction (EBSD) has developed over the last few decades into a valuable crystallographic characterisation method for a wide range of sample types. Despite these advances, issues such as the complexity of sample preparation, relatively slow acquisition, and damage in beam-sensitive samples, still limit the quantity and quality of interpretable data that can be obtained. To mitigate these issues, here we propose a method based on the subsampling of probe positions and subsequent reconstruction of an incomplete data set. The missing probe locations (or pixels in the image) are recovered via an inpainting process using a dictionary-learning based method called beta-process factor analysis (BPFA). To investigate the robustness of both our inpainting method and Hough-based indexing, we simulate subsampled and noisy EBSD data sets from a real fully sampled Ni-superalloy data set for different subsampling ratios of probe positions using both Gaussian and Poisson noise models. We find that zero solution pixel detection (inpainting un-indexed pixels) enables higher-quality reconstructions to be obtained. Numerical tests confirm high-quality reconstruction of band contrast and inverse pole figure maps from only 10% of the probe positions, with the potential to reduce this to 5% if only inverse pole figure maps are needed. These results show the potential application of this method in EBSD, allowing for faster analysis and extending the use of this technique to beam sensitive materials.

摘要

电子背散射衍射(EBSD)在过去几十年中已发展成为一种适用于多种样品类型的有价值的晶体学表征方法。尽管取得了这些进展,但诸如样品制备复杂、采集相对较慢以及对束敏感样品造成损伤等问题,仍然限制了可获得的可解释数据的数量和质量。为了缓解这些问题,我们在此提出一种基于对探测位置进行子采样并随后重建不完整数据集的方法。缺失的探测位置(或图像中的像素)通过使用一种基于字典学习的方法——贝塔过程因子分析(BPFA)的修复过程来恢复。为了研究我们的修复方法和基于霍夫的索引的稳健性,我们使用高斯和泊松噪声模型,从一个真实的全采样镍基高温合金数据集中模拟不同探测位置子采样率的子采样和噪声EBSD数据集。我们发现零解像素检测(修复未索引像素)能够获得更高质量的重建。数值测试证实,仅从10%的探测位置就能高质量重建带衬度和反极图,若仅需要反极图,有可能将此比例降至5%。这些结果表明了该方法在EBSD中的潜在应用,可实现更快的分析,并将该技术的应用扩展到对束敏感的材料。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2f22/11891967/66a8e0896108/JMI-298-44-g009.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2f22/11891967/66a8e0896108/JMI-298-44-g009.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2f22/11891967/66a8e0896108/JMI-298-44-g009.jpg

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本文引用的文献

1
High-speed 4-dimensional scanning transmission electron microscopy using compressive sensing techniques.使用压缩传感技术的高速四维扫描透射电子显微镜。
J Microsc. 2024 Sep;295(3):278-286. doi: 10.1111/jmi.13315. Epub 2024 May 6.
2
The Potential of Subsampling and Inpainting for Fast Low-Dose Cryo FIB-SEM Imaging.子采样和图像修复在快速低剂量冷冻聚焦离子束扫描电子显微镜成像中的潜力
Microsc Microanal. 2024 Mar 7;30(1):96-102. doi: 10.1093/micmic/ozae005.
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High-throughput determination of grain size distributions by EBSD with low-discrepancy sampling.
J Microsc. 2024 Jan;293(1):20-37. doi: 10.1111/jmi.13247. Epub 2023 Dec 18.
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Demonstration of an AI-driven workflow for autonomous high-resolution scanning microscopy.人工智能驱动的自主高分辨率扫描显微镜工作流程展示。
Nat Commun. 2023 Sep 7;14(1):5501. doi: 10.1038/s41467-023-40339-1.
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Towards real-time STEM simulations through targeted subsampling strategies.
J Microsc. 2023 Apr;290(1):53-66. doi: 10.1111/jmi.13177. Epub 2023 Feb 27.
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SIM-STEM Lab: Incorporating Compressed Sensing Theory for Fast STEM Simulation.SIM-STEM实验室:融合压缩感知理论以实现快速STEM模拟。
Ultramicroscopy. 2022 Dec;242:113625. doi: 10.1016/j.ultramic.2022.113625. Epub 2022 Sep 25.
7
Sub-Sampled Imaging for STEM: Maximising Image Speed, Resolution and Precision Through Reconstruction Parameter Refinement.用于扫描透射电子显微镜的子采样成像:通过重建参数优化实现图像速度、分辨率和精度的最大化
Ultramicroscopy. 2022 Mar;233:113451. doi: 10.1016/j.ultramic.2021.113451. Epub 2021 Dec 7.
8
Electron backscattered diffraction using a new monolithic direct detector: High resolution and fast acquisition.使用新型单片式直接探测器的电子背散射衍射:高分辨率与快速采集。
Ultramicroscopy. 2021 Jan;220:113160. doi: 10.1016/j.ultramic.2020.113160. Epub 2020 Nov 4.
9
A spherical harmonic transform approach to the indexing of electron back-scattered diffraction patterns.一种用于电子背散射衍射图案索引的球谐变换方法。
Ultramicroscopy. 2019 Dec;207:112841. doi: 10.1016/j.ultramic.2019.112841. Epub 2019 Sep 3.
10
NLPAR: Non-local smoothing for enhanced EBSD pattern indexing.
Ultramicroscopy. 2019 May;200:50-61. doi: 10.1016/j.ultramic.2019.02.013. Epub 2019 Feb 19.