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用于提高采收率的氨基酸离子液体的合成与评价：实验与模型模拟研究

Synthesis and evaluation of amino acid ionic liquid for enhanced oil recovery: experimental and modeling simulation studies.

作者信息

Mansour E M, Hosny R, Mohamed Ammona S, Abdelhafiz Fatma M

机构信息

PVT Lab, Production Department, Egyptian Petroleum Research Institute, 1 Ahmed El Zomor St., Nasr City, Cairo, 11727, Egypt.

PVT Services Center, Egyptian Petroleum Research Institute, 1 Ahmed El Zomor St., Nasr City, Cairo, 11727, Egypt.

出版信息

Sci Rep. 2025 Jan 16;15(1):2201. doi: 10.1038/s41598-025-85560-8.

DOI:10.1038/s41598-025-85560-8
PMID:39820535
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11739425/
Abstract

Recovering the remaining oil after primary and secondary extraction methods poses a significant challenge. Enhanced oil recovery (EOR) techniques, which involve injecting fluids into reservoirs, aim to increase recovery rates. Ionic liquids, known for their adaptability, are emerging as promising agents in EOR, improving oil displacement by reshaping fluid properties and interacting with reservoir rocks. This study investigates the eco-friendly amino acid ionic liquid, AAIL [G0.5 C12][Pro], for EOR applications, focusing on its characterization and performance. Using pre-prepared quaternary ammonium salt PAMAM G0.5 C12 and proline, AAIL [G0.5 C12][Pro] was synthesized and confirmed via FTIR and 1H-NMR analyses. Rheological analysis identified 7 g of AAIL [G0.5 C12][Pro] as the optimal concentration for peak performance. Laboratory sand-pack displacement experiments demonstrated an 11% increase in oil recovery at this concentration. Further, a 3D reservoir model simulation validated the enhanced oil recovery potential of AAIL [G0.5 C12][Pro]. The study introduces the novel amino acid ionic liquid [G0.5 C12][Pro], which demonstrates superior effectiveness in enhancing oil recovery through significant wettability modification and interfacial tension reduction, underscoring its potential as an effective and environmentally friendly EOR agent compared to other ionic liquids and conventional methods.

摘要

在一次和二次采油方法之后回收剩余原油是一项重大挑战。强化采油（EOR）技术，即向油藏注入流体，旨在提高采收率。离子液体以其适应性著称，正成为EOR中有前景的试剂，通过重塑流体性质和与油藏岩石相互作用来改善驱油效果。本研究调查了用于EOR应用的环保型氨基酸离子液体AAIL [G0.5 C12][Pro]，重点关注其表征和性能。使用预先制备的季铵盐PAMAM G0.5 C12和脯氨酸，合成了AAIL [G0.5 C12][Pro]，并通过傅里叶变换红外光谱（FTIR）和核磁共振氢谱（1H-NMR）分析进行了确认。流变学分析确定7克AAIL [G0.5 C12][Pro]为实现最佳性能的最佳浓度。实验室填砂驱替实验表明，在此浓度下，采收率提高了11%。此外，三维油藏模型模拟验证了AAIL [G0.5 C12][Pro]提高采收率的潜力。该研究引入了新型氨基酸离子液体[G0.5 C12][Pro]，它通过显著改变润湿性和降低界面张力，在提高采收率方面显示出卓越的效果，突出了其与其他离子液体和传统方法相比，作为一种有效且环保的EOR试剂的潜力。

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