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通过跨尺度模式耦合到WSe薄膜中的纳米机械共振来动态调谐太赫兹原子晶格振动

Dynamic tuning of terahertz atomic lattice vibration via cross-scale mode coupling to nanomechanical resonance in WSe membranes.

作者信息

Xu Bo, Zhang Zejuan, Qin Jiaze, Wu Jiaqi, Wang Luming, Zhu Jiankai, Jiao Chenyin, Zhang Wanli, Xia Juan, Wang Zenghui

机构信息

Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu, 610054, China.

Hubei Key Laboratory of Micro-Nanoelectronic Materials and Devices, Hubei University, Wuhan, 430062, China.

出版信息

Microsyst Nanoeng. 2025 Jan 22;11(1):18. doi: 10.1038/s41378-024-00827-w.

DOI:10.1038/s41378-024-00827-w
PMID:39843422
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11754608/
Abstract

Nanoelectromechanical systems (NEMS) based on atomically-thin tungsten diselenide (WSe), benefiting from the excellent material properties and the mechanical degree of freedom, offer an ideal platform for studying and exploiting dynamic strain engineering and cross-scale vibration coupling in two-dimensional (2D) crystals. However, such opportunity has remained largely unexplored for WSe NEMS, impeding exploration of exquisite physical processes and realization of novel device functions. Here, we demonstrate dynamic coupling between atomic lattice vibration and nanomechanical resonances in few-layer WSe NEMS. Using a custom-built setup capable of simultaneously detecting Raman and motional signals, we accomplish cross-scale mode coupling between the THz crystal phonon and MHz structural vibration, achieving GHz frequency tuning in the atomic lattice modes with a dynamic gauge factor of 61.9, the best among all 2D crystals reported to date. Our findings show that such 2D NEMS offer great promises for exploring cross-scale physics in atomically-thin semiconductors.

摘要

基于原子级薄的二硒化钨(WSe₂)的纳米机电系统(NEMS),受益于其优异的材料特性和机械自由度,为研究和利用二维(2D)晶体中的动态应变工程及跨尺度振动耦合提供了一个理想平台。然而,对于WSe₂ NEMS而言,这样的机会在很大程度上仍未得到探索,这阻碍了对精细物理过程的探究以及新型器件功能的实现。在此,我们展示了少层WSe₂ NEMS中原子晶格振动与纳米机械共振之间的动态耦合。通过使用能够同时检测拉曼信号和运动信号的定制装置,我们实现了太赫兹(THz)晶体声子与兆赫兹(MHz)结构振动之间的跨尺度模式耦合,在原子晶格模式中实现了吉赫兹(GHz)频率调谐,动态应变系数为61.9,这是迄今为止所有已报道的二维晶体中最佳的。我们的研究结果表明,此类二维NEMS在探索原子级薄半导体中的跨尺度物理方面具有巨大潜力。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/05e4/11754608/72a4e397ebb8/41378_2024_827_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/05e4/11754608/3d0f05c4cb0c/41378_2024_827_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/05e4/11754608/90c542297ccb/41378_2024_827_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/05e4/11754608/07a9ad0b2945/41378_2024_827_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/05e4/11754608/72a4e397ebb8/41378_2024_827_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/05e4/11754608/3d0f05c4cb0c/41378_2024_827_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/05e4/11754608/90c542297ccb/41378_2024_827_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/05e4/11754608/07a9ad0b2945/41378_2024_827_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/05e4/11754608/72a4e397ebb8/41378_2024_827_Fig4_HTML.jpg

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本文引用的文献

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Identifying, Resolving, and Quantifying Anisotropy in ReS Nanomechanical Resonators.识别、解决和量化 ReS 纳米机械谐振器中的各向异性。
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Electrically Tunable MXene Nanomechanical Resonators Vibrating at Very High Frequencies.电调谐MXene纳米机械谐振器在甚高频下振动。
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Frequency Scaling, Elastic Transition, and Broad-Range Frequency Tuning in WSe Nanomechanical Resonators.WSe 纳米机械谐振器中的频率缩放、弹性转变和宽范围频率调谐
Nano Lett. 2022 Jul 13;22(13):5107-5113. doi: 10.1021/acs.nanolett.2c00494. Epub 2022 May 6.
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