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多功能生物材料BTO/Ag的简便制备及其在光电化学传感、光降解和抗菌活性方面的应用。

Facile preparation of multifunctional biomaterials BTO/Ag and their applications in photoelectrochemical sensing, photodegradation and antibacterial activities.

作者信息

Kexi Zhang, Bingdong Yan, Delun Chen, Xiaohong Wang, Yang Cao, Xuewei Zhang, Wanjun Hao, Jinchun Tu

机构信息

College of Material Science and Engineering, Key Laboratory of Advanced Materials of Tropical Island Resources, Ministry of Education, Hainan University Haikou 570228 China

Key Laboratory of Child Cognition and Behavior Development of Hainan Province, Qiongtai Normal University Haikou 571100 China.

出版信息

RSC Adv. 2025 Jan 27;15(4):2657-2667. doi: 10.1039/d4ra07385a. eCollection 2025 Jan 23.

DOI:10.1039/d4ra07385a
PMID:39871978
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11770675/
Abstract

With the progress of modern technology and the diversification of societal demands, traditional materials with single properties can no longer meet the requirements of complex and constantly evolving application scenarios. To tackle intricate biomedical applications like disease diagnosis and treatment, scientists are focusing on exploring the design of novel multifunctional biomaterials that possess diverse activities. Bismuth titanate (BiTiO, BTO), which has multifunctionality and great application potential, unfortunately suffers from inadequate photocatalytic performance. On the other hand, silver nanoparticles (Ag), known for their antibacterial properties, have relatively limited functions. In this study, we overcame these limitations by combining BTO with Ag to form a BTO/Ag biomultifunctional material. Our experiments showed that the addition of Ag effectively improved BTO's UV absorption ability, decreased electron transfer resistance, and increased carrier concentration. As a result, the photocatalytic performance of BTO/Ag was significantly enhanced, and its photoelectrochemical sensing and photodegradation capabilities were also greatly improved. Moreover, BTO served as an effective substrate, preventing Ag from agglomerating and maximizing its antibacterial potential. In specific performance evaluations, ascorbic acid and methylene blue (MB) were used to study the photoelectrochemical sensing and photodegradation capabilities respectively, while and were chosen as test organisms to assess the antibacterial properties. All in all, this research has yielded promising results.

摘要

随着现代技术的进步和社会需求的多样化,具有单一性能的传统材料已无法满足复杂且不断演变的应用场景的要求。为了应对疾病诊断和治疗等复杂的生物医学应用,科学家们正专注于探索具有多种活性的新型多功能生物材料的设计。钛酸铋(BiTiO,BTO)具有多功能性和巨大的应用潜力,但不幸的是其光催化性能不足。另一方面,以抗菌性能闻名的银纳米颗粒(Ag)功能相对有限。在本研究中,我们通过将BTO与Ag结合形成BTO/Ag生物多功能材料克服了这些局限性。我们的实验表明,Ag的添加有效提高了BTO的紫外吸收能力,降低了电子转移电阻,并增加了载流子浓度。结果,BTO/Ag的光催化性能显著增强,其光电化学传感和光降解能力也大大提高。此外,BTO作为有效的基底,防止Ag团聚并使其抗菌潜力最大化。在具体性能评估中,分别使用抗坏血酸和亚甲基蓝(MB)研究光电化学传感和光降解能力,同时选择 和 作为测试生物体来评估抗菌性能。总而言之,这项研究取得了有前景的结果。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/3667a7ce34b2/d4ra07385a-f9.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/d77677a54776/d4ra07385a-s1.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/92018ae62a99/d4ra07385a-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/21e971201367/d4ra07385a-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/2dd6f81bd4b8/d4ra07385a-f7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/6f7281de76ac/d4ra07385a-f8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/3667a7ce34b2/d4ra07385a-f9.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/d77677a54776/d4ra07385a-s1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/fde2add93649/d4ra07385a-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/9fb775215f45/d4ra07385a-f2.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/cb1e466158af/d4ra07385a-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/92018ae62a99/d4ra07385a-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/21e971201367/d4ra07385a-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/2dd6f81bd4b8/d4ra07385a-f7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/6f7281de76ac/d4ra07385a-f8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a079/11770675/3667a7ce34b2/d4ra07385a-f9.jpg

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