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利用高分辨率卫星反演的一氧化氮(NO)估计值评估一氧化氮暴露代表性和社会经济差异。

Leveraging High-Resolution Satellite-Derived NO Estimates to Evaluate NO Exposure Representativeness and Socioeconomic Disparities.

作者信息

Kim Na Rae, Lee Hyung Joo

机构信息

Division of Environmental Science and Engineering, Pohang University of Science and Technology (POSTECH), Pohang, Gyeongbuk 37673, Republic of Korea.

Institute for Convergence Research and Education in Advanced Technology, Yonsei University, Incheon 21983, Republic of Korea.

出版信息

Environ Sci Technol. 2025 Feb 25;59(7):3434-3442. doi: 10.1021/acs.est.4c10996. Epub 2025 Feb 13.

DOI:10.1021/acs.est.4c10996
PMID:39947832
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11866924/
Abstract

Research has typically estimated NO concentrations over several kilometers; thus, NO data at finer spatial resolution remain limited. This study used tropospheric NO data from the TROPOspheric Monitoring Instrument (TROPOMI) and traffic-related land use parameters to estimate long-term average NO concentrations at a spatial resolution of 500 m in South Korea from 2018 to 2022. Our satellite-land use hybrid regression model showed reasonably high predictability with a cross-validation of 0.81, mean absolute error of 2.28 ppb and root mean squared error of 2.85 ppb. Leveraging these high-resolution data, we assessed the representativeness of ground monitors for population exposure by comparing population-weighted NO concentrations from estimated and measured data. Across 17 metropolitan cities and provinces, the ratios of population-weighted estimated to measured NO ranged from 0.62 to 1.12, with the ratio of 1 exhibiting the most representative monitoring networks. We further investigated disproportionate NO exposures based on socioeconomic status, revealing that NO exposures were consistently higher in local districts with higher socioeconomic status because of the unique historical backgrounds of rapid economic development and urban infrastructure design in South Korea. Using high-resolution NO data can lead to more comprehensive and precise exposure assessments, enhancing public health and regulatory applications.

摘要

研究通常估算的是数公里范围内的一氧化氮(NO)浓度;因此,空间分辨率更高的NO数据仍然有限。本研究使用了对流层监测仪器(TROPOMI)的对流层NO数据以及与交通相关的土地利用参数,来估算2018年至2022年韩国500米空间分辨率下的长期平均NO浓度。我们的卫星-土地利用混合回归模型显示出相当高的预测能力,交叉验证值为0.81,平均绝对误差为2.28 ppb,均方根误差为2.85 ppb。利用这些高分辨率数据,我们通过比较估算数据和实测数据的人口加权NO浓度,评估了地面监测站对人群暴露的代表性。在17个大城市和省份中,人口加权估算NO与实测NO的比值在0.62至1.12之间,比值为1时表示监测网络最具代表性。我们还根据社会经济地位调查了不成比例的NO暴露情况,结果显示,由于韩国经济快速发展和城市基础设施设计的独特历史背景,社会经济地位较高的地区的NO暴露一直较高。使用高分辨率的NO数据可以进行更全面、精确的暴露评估,加强公共卫生和监管应用。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1094/11866924/7a011dea5864/es4c10996_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1094/11866924/2b4b62d10a2d/es4c10996_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1094/11866924/72620083717e/es4c10996_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1094/11866924/7a011dea5864/es4c10996_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1094/11866924/2b4b62d10a2d/es4c10996_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1094/11866924/72620083717e/es4c10996_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1094/11866924/7a011dea5864/es4c10996_0003.jpg

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本文引用的文献

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Sci Total Environ. 2023 Jan 20;857(Pt 3):159342. doi: 10.1016/j.scitotenv.2022.159342. Epub 2022 Oct 9.
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Historical Redlining Is Associated with Present-Day Air Pollution Disparities in U.S. Cities.历史上的红线划定与美国城市当今的空气污染差异有关。
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Air pollution exposure disparities across US population and income groups.
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Short term associations of ambient nitrogen dioxide with daily total, cardiovascular, and respiratory mortality: multilocation analysis in 398 cities.短期环境二氧化氮与每日全因、心血管和呼吸死亡率的关联:398 个城市的多地点分析。
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Spatiotemporal mapping and assessment of daily ground NO concentrations in China using high-resolution TROPOMI retrievals.利用高分辨率TROPOMI反演数据对中国地面每日一氧化氮浓度进行时空映射与评估
Environ Pollut. 2021 Jan 8;273:116456. doi: 10.1016/j.envpol.2021.116456.
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Enhanced Capabilities of TROPOMI NO: Estimating NO from North American Cities and Power Plants.TROPOMI 硝酸盐观测能力增强:估算北美城市和发电厂的氮氧化物。
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