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扭曲双层MoSe₂中广义电子晶体的量子熔化

Quantum melting of generalized electron crystal in twisted bilayer MoSe.

作者信息

Zong Qi Jun, Wang Haolin, Zhang Qi, Cheng Xinle, He Yangchen, Xu Qiaoling, Fischer Ammon, Watanabe Kenji, Taniguchi Takashi, Rhodes Daniel A, Xian Lede, Kennes Dante M, Rubio Angel, Yu Geliang, Wang Lei

机构信息

National Laboratory of Solid-State Microstructures, School of Physics and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, China.

School of Advanced Materials and Nanotechnology, Xidian University, Xi'an, China.

出版信息

Nat Commun. 2025 Apr 30;16(1):4058. doi: 10.1038/s41467-025-59365-2.

DOI:10.1038/s41467-025-59365-2
PMID:40307227
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12044088/
Abstract

Electrons can form an ordered solid crystal phase ascribed to the interplay between Coulomb repulsion and kinetic energy. Tuning these energy scales can drive a phase transition from electron solid to liquid, i.e., melting of Wigner crystal. Generalized Wigner crystals (GWCs) pinned to moiré superlattices have been reported by optical and scanning-probe-based methods. Using transport measurements to investigate GWCs is vital to a complete characterization, however, still poses a significant challenge due to difficulties in making reliable electrical contacts. Here, we report the electrical transport detection of GWCs at fractional fillings ν = 2/5, 1/2, 3/5, 2/3, 8/9, 10/9, and 4/3 in twisted bilayer MoSe. We further observe that these GWCs undergo continuous quantum melting transitions to liquid phases by tuning doping density, magnetic and displacement fields, manifested by quantum critical scaling behaviors. Our findings establish twisted bilayer MoSe as a novel system to study strongly correlated states of matter and their quantum phase transitions.

摘要

电子可以形成一种有序的固体晶体相,这归因于库仑排斥力和动能之间的相互作用。调节这些能量尺度可以驱动从电子固体到液体的相变,即维格纳晶体的熔化。通过基于光学和扫描探针的方法,已经报道了固定在莫尔超晶格上的广义维格纳晶体(GWC)。然而,使用输运测量来研究GWC对于完整表征至关重要,但由于难以制作可靠的电接触,这仍然是一个重大挑战。在这里,我们报告了在扭曲双层MoSe中分数填充ν = 2/5、1/2、3/5、2/3、8/9、10/9和4/3时GWC的电输运检测。我们进一步观察到,通过调节掺杂密度、磁场和位移场,这些GWC经历连续的量子熔化转变为液相,表现为量子临界标度行为。我们的发现将扭曲双层MoSe确立为研究强关联物质状态及其量子相变的新型系统。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/978b/12044088/ef65137bd28a/41467_2025_59365_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/978b/12044088/e103c7a60097/41467_2025_59365_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/978b/12044088/5b5b02533892/41467_2025_59365_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/978b/12044088/ccbdff7ce4b6/41467_2025_59365_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/978b/12044088/ef65137bd28a/41467_2025_59365_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/978b/12044088/e103c7a60097/41467_2025_59365_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/978b/12044088/5b5b02533892/41467_2025_59365_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/978b/12044088/ccbdff7ce4b6/41467_2025_59365_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/978b/12044088/ef65137bd28a/41467_2025_59365_Fig4_HTML.jpg

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本文引用的文献

1
Quantum Melting of Generalized Wigner Crystals in Transition Metal Dichalcogenide Moiré Systems.过渡金属二硫属化物莫尔系统中广义维格纳晶体的量子熔化
Phys Rev Lett. 2024 Oct 11;133(15):156501. doi: 10.1103/PhysRevLett.133.156501.
2
Wigner molecular crystals from multielectron moiré artificial atoms.来自多电子莫尔人造原子的维格纳分子晶体。
Science. 2024 Jul 5;385(6704):86-91. doi: 10.1126/science.adk1348. Epub 2024 Jul 4.
3
Direct observation of a magnetic-field-induced Wigner crystal.磁场诱导威格纳晶体的直接观察。
Nature. 2024 Apr;628(8007):287-292. doi: 10.1038/s41586-024-07212-7. Epub 2024 Apr 10.
4
Mapping charge excitations in generalized Wigner crystals.广义维格纳晶体中的电荷激发映射
Nat Nanotechnol. 2024 May;19(5):618-623. doi: 10.1038/s41565-023-01594-x. Epub 2024 Jan 29.
5
Giant Correlated Gap and Possible Room-Temperature Correlated States in Twisted Bilayer MoS_{2}.扭曲双层二硫化钼中的巨大关联能隙和可能的室温关联态
Phys Rev Lett. 2023 Dec 22;131(25):256201. doi: 10.1103/PhysRevLett.131.256201.
6
Moving Crystal Phases of a Quantum Wigner Solid in an Ultra-High-Quality 2D Electron System.高质量二维电子系统中量子维格纳晶体的移动晶相
Phys Rev Lett. 2023 Dec 8;131(23):236501. doi: 10.1103/PhysRevLett.131.236501.
7
Magnetic Field-Stabilized Wigner Crystal States in a Graphene Moiré Superlattice.石墨烯莫尔超晶格中的磁场稳定维格纳晶体态
Nano Lett. 2023 Aug 9;23(15):7023-7028. doi: 10.1021/acs.nanolett.3c01741. Epub 2023 Jul 20.
8
Tunable spin and valley excitations of correlated insulators in Γ-valley moiré bands.Γ 谷摩尔带关联绝缘体内可调谐的自旋和谷激发。
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Melting of generalized Wigner crystals in transition metal dichalcogenide heterobilayer Moiré systems.过渡金属二硫属化物异质双层莫尔系统中广义维格纳晶体的熔化
Nat Commun. 2022 Nov 19;13(1):7098. doi: 10.1038/s41467-022-34683-x.
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Nat Commun. 2022 Jul 25;13(1):4271. doi: 10.1038/s41467-022-32037-1.