Zhang Qianpeng, Sun Xiaofei, Chen Guanyu, Ma Zichao, Zhang Daquan, Zhou Yu, Qiu Xiao, Ren Beitao, Ding Yucheng, Poddar Swapnadeep, Tang Wenying, Lv Hualiang, Mo Xiaoliang, Fan Zhiyong
State Key Laboratory of Photovoltaic Science and Technology, Shanghai Frontiers Science Research Base of Intelligent Optoelectronics and Perception, Institute of Optoelectronics, Fudan University, Shanghai 200433, China.
Department of Electronic and Computer Engineering, State Key Laboratory of Advanced Displays and Optoelectronics Technologies, The Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong SAR, China.
Sci Adv. 2025 May 16;11(20):eadu3840. doi: 10.1126/sciadv.adu3840. Epub 2025 May 14.
Halide perovskite materials excel in broad optoelectronic applications, and there is an urgent demand to develop perovskite-based integrated optoelectronic devices. However, the limitations posed by the incompatibility of perovskite thin film with wet lithography greatly hinder its potential in many important applications, including ultrahigh-density displays, high-resolution image sensors, high-density memristors, and integrated photonic circuitry. To tackle this bottleneck problem, we develop the self-aligned close-spaced sublimation growth of perovskite quantum wires and demonstrate 0.18-micrometer feature size perovskite patterns, meanwhile achieving a pixel density of 63,500 pixels per inch, the highest reported for perovskite. We showcase pixelation of perovskite quantum wires with color conversion films, addressing the need for full-color microdisplays. In addition, we demonstrate these films on curved substrates, holding promise for near-eye microdisplays. Processes shown here can also apply to other perovskite devices such as high-resolution displays, image sensing, and memristor arrays.
卤化物钙钛矿材料在广泛的光电子应用中表现出色,因此迫切需要开发基于钙钛矿的集成光电器件。然而,钙钛矿薄膜与湿法光刻不兼容所带来的限制极大地阻碍了其在许多重要应用中的潜力,包括超高密度显示器、高分辨率图像传感器、高密度忆阻器和集成光子电路。为了解决这一瓶颈问题,我们开发了钙钛矿量子线的自对准近距离升华生长,并展示了特征尺寸为0.18微米的钙钛矿图案,同时实现了每英寸63,500像素的像素密度,这是钙钛矿报道的最高值。我们展示了带有颜色转换膜的钙钛矿量子线像素化,满足了全彩微型显示器的需求。此外,我们在弯曲基板上展示了这些薄膜,有望用于近眼微型显示器。这里展示的工艺也可应用于其他钙钛矿器件,如高分辨率显示器、图像传感和忆阻器阵列。