Deng Qiyu, Zhu Hengjia, Zhao Zhipeng, Li Hegeng, Yang Ling, Wu Xinya, Zhang Yiyuan, Yu Peng, Tang Xin, Li Wei, Yin Xiaobo, Wang Liqiu
Department of Mechanical Engineering, The University of Hong Kong, Hong Kong SAR, PR China.
Department of Mechanical Engineering, The Hong Kong Polytechnic University, Hong Kong SAR, PR China.
Nat Commun. 2025 May 17;16(1):4601. doi: 10.1038/s41467-025-59663-9.
Adjusting magnetization orienting and conformal assembling of high-coercivity micro-magnets at the microscale remains challenging, despite long-standing demand for space-resolved magnetic modulation in various applications. Local magnetic modulation, including remagnetization or reassembly, typically requires high fields and temperatures to overcome the coercivity and stringent conditions while suffering from low assembly efficiency or poor spatial resolution. Here, we report a linear magnet composed of a hydrogel (alginate) matrix and precisely discrete phase-change-material (PCM, eicosane) cells containing micro-magnetic particles (NdFeB, 5 µm). Moderate local laser heating (40 °C) reversibly switches PCM from solid to fluid state thus relaxing particles' interfacial constraints inside the hydrogel matrix, overcoming the high-coercivity of magnetic assembly and allowing particles in cells to reorient under mild fields (≤30 mT). The linear magnet shows excellent discrete magnetization programmability (~150 µm) and stretchability (strain ~80%), enabling versatile functionalities such as conformal and patterned field generation, soft robotic actuation, flexible sensing, and interactive wearables with dynamically coded information.
尽管在各种应用中对空间分辨磁调制的需求由来已久,但在微观尺度上调整高矫顽力微磁体的磁化方向和共形组装仍然具有挑战性。局部磁调制,包括再磁化或重新组装,通常需要高场和高温来克服矫顽力和严格的条件,同时存在组装效率低或空间分辨率差的问题。在这里,我们报道了一种由水凝胶(藻酸盐)基质和精确离散的相变材料(PCM,二十烷)单元组成的线性磁体,这些单元包含微磁性颗粒(钕铁硼,5 µm)。适度的局部激光加热(40 °C)可使PCM可逆地从固态转变为液态,从而缓解水凝胶基质内颗粒的界面约束,克服磁组装的高矫顽力,并允许单元内的颗粒在弱磁场(≤30 mT)下重新定向。该线性磁体具有出色的离散磁化可编程性(150 µm)和拉伸性(应变80%),能够实现多种功能,如共形和图案化场生成、软机器人驱动、柔性传感以及具有动态编码信息的交互式可穿戴设备。