Morano V C, Maesen Z, Nikitin S E, Lass J, Mazzone D G, Zaharko O
PSI, Center for Neutron and Muon Sciences, Forschungsstrasse 111, 5232 Villigen, PSI, Switzerland.
Phys Rev Lett. 2025 Jun 6;134(22):226702. doi: 10.1103/PhysRevLett.134.226702.
Altermagnets are collinear compensated magnets in which the magnetic sublattices are related by rotation rather than translation or inversion. One of the quintessential properties of altermagnets is the presence of split chiral magnon modes. Recently, such modes have been predicted in MnF_{2}. Here, we report inelastic neutron scattering results on an MnF_{2} single crystal along high-symmetry Brillouin zone paths for which the magnon splitting is expected. Within the resolution of our measurement, we do not observe the predicted splitting. The inelastic spectrum is well modeled using J_{1}, J_{2}, J_{3} nearest-neighbor exchange interactions with weak uniaxial anisotropy. These interactions have higher symmetry than the crystal lattice, while the interactions predicted to produce the altermagnetic splitting are negligibly small. Therefore, the two magnon modes appear to be degenerate over the entire Brillouin zone and the spin dynamics of MnF_{2} is indistinguishable from a classical Néel antiferromagnet. Application of a magnetic field causes a Zeeman splitting of the magnon modes close to the Γ point. Even if chiral magnon modes are allowed by altermagnetic symmetry, the splitting in real materials such as MnF_{2} can be negligibly small.
交替磁体是共线补偿磁体,其中磁亚晶格通过旋转而非平移或反演相关联。交替磁体的一个典型特性是存在分裂手性磁振子模式。最近,在氟化锰(MnF₂)中预测到了这种模式。在此,我们报告了沿高对称布里渊区路径对MnF₂单晶进行非弹性中子散射的结果,预计在此路径上会出现磁振子分裂。在我们的测量分辨率范围内,我们未观察到预测的分裂。使用具有弱单轴各向异性的J₁、J₂、J₃最近邻交换相互作用对非弹性谱进行了很好的建模。这些相互作用比晶格具有更高的对称性,而预计会产生交替磁分裂的相互作用小到可以忽略不计。因此,这两种磁振子模式在整个布里渊区似乎是简并的,并且MnF₂的自旋动力学与经典尼尔反铁磁体无法区分。施加磁场会导致靠近Γ点的磁振子模式发生塞曼分裂。即使交替磁对称性允许手性磁振子模式存在,但在诸如MnF₂等实际材料中的分裂可能小到可以忽略不计。