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用于色散样品的超宽带叠层成像术

Ultra-broadband ptychography for dispersive samples.

作者信息

Lin Huixiang, Lin Angyi, Jin Xiaoyu, Li Kui, Niu Jin, Li Jie, Zhang Xiaoshi, Liu Tao, Xu Wenhui, Zhang Fucai

机构信息

State Key Laboratory of Quantum Functional Materials, Department of Electronic and Electrical Engineering, Southern University of Science and Technology, Shenzhen, China.

School of Physics and Astronomy, Yunnan University, Kunming, Yunnan, China.

出版信息

Nat Commun. 2025 Jul 1;16(1):5714. doi: 10.1038/s41467-025-61339-3.

DOI:10.1038/s41467-025-61339-3
PMID:40592847
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12215532/
Abstract

X-ray ptychography has emerged as a powerful imaging tool on X-ray synchrotron facilities. Implementation of ptychography on laboratory-scale X-ray sources has largely been hindered by their poor temporal coherence and low flux. Here we propose an ultra-broadband method incorporating structured illumination to enhance the robustness of ptychography to broadband sources. Different from other methods, our ultra-broadband ptychography method enables imaging of dispersive samples without prior knowledge of light spectra. A 60% bandwidth light source and a high harmonic extreme ultraviolet source were used to validate our method. Moreover, our method demonstrates precise quantitative phase imaging capabilities. The proposed method will significantly advance the implementation of ptychography on laboratory-scale broadband X-ray sources and widen its applications in biomedicine and materials science.

摘要

X射线叠层成像术已成为X射线同步辐射装置上一种强大的成像工具。在实验室规模的X射线源上实施叠层成像术很大程度上受到其时间相干性差和通量低的阻碍。在此,我们提出一种结合结构化照明的超宽带方法,以增强叠层成像术对宽带源的鲁棒性。与其他方法不同,我们的超宽带叠层成像术方法能够在无需光光谱先验知识的情况下对色散样品进行成像。使用了一个60%带宽的光源和一个高次谐波极紫外光源来验证我们的方法。此外,我们的方法展示了精确的定量相位成像能力。所提出的方法将显著推动叠层成像术在实验室规模宽带X射线源上的实施,并拓宽其在生物医学和材料科学中的应用。

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本文引用的文献

1
A high-performance reconstruction method for partially coherent ptychography.
Ultramicroscopy. 2024 Dec;267:114068. doi: 10.1016/j.ultramic.2024.114068. Epub 2024 Oct 28.
2
Ultra-broadband diffractive imaging with unknown probe spectrum.具有未知探测光谱的超宽带衍射成像
Light Sci Appl. 2024 Aug 26;13(1):213. doi: 10.1038/s41377-024-01581-4.
3
Wavelength-multiplexed multi-mode EUV reflection ptychography based on automatic differentiation.基于自动微分的波长复用多模极紫外反射叠层成像技术
Light Sci Appl. 2024 Aug 19;13(1):196. doi: 10.1038/s41377-024-01558-3.
4
High-performance 4-nm-resolution X-ray tomography using burst ptychography.利用爆发式叠层相位成像术实现高性能 4nm 分辨率 X 射线断层摄影。
Nature. 2024 Aug;632(8023):81-88. doi: 10.1038/s41586-024-07615-6. Epub 2024 Jul 31.
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Broadband coherent modulation imaging with no knowledge of the illumination spectrum distribution.在不了解照明光谱分布的情况下进行宽带相干调制成像。
Opt Lett. 2023 Aug 1;48(15):3977-3980. doi: 10.1364/OL.495706.
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Material-specific high-resolution table-top extreme ultraviolet microscopy.特定材料的高分辨率桌面式极紫外显微镜。
Light Sci Appl. 2022 Apr 29;11(1):117. doi: 10.1038/s41377-022-00797-6.
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Numerical and experimental study of partial coherence for near-field and far-field ptychography.近场和远场叠层成像术的部分相干性的数值与实验研究。
Opt Express. 2021 Nov 22;29(24):40652-40667. doi: 10.1364/OE.445978.
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X-Ray Ptychography with a Laboratory Source.实验室光源的 X 射线叠层成像技术。
Phys Rev Lett. 2021 May 14;126(19):193902. doi: 10.1103/PhysRevLett.126.193902.
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Nondestructive, high-resolution, chemically specific 3D nanostructure characterization using phase-sensitive EUV imaging reflectometry.使用相敏极紫外成像反射测量法进行无损、高分辨率、化学特异性的三维纳米结构表征。
Sci Adv. 2021 Jan 27;7(5). doi: 10.1126/sciadv.abd9667. Print 2021 Jan.
10
Broadband X-ray ptychography using multi-wavelength algorithm.使用多波长算法的宽带X射线叠层成像术
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