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通过共振非弹性X射线散射观测自旋流差异

Observing differential spin currents by resonant inelastic X-ray scattering.

作者信息

Gu Yanhong, Barker Joseph, Li Jiemin, Kikkawa Takashi, Camino Fernando, Kisslinger Kim, Sinsheimer John, Lienhard Lukas, Bauer Jackson J, Ross Caroline A, Basov Dmitri N, Saitoh Eiji, Pelliciari Jonathan, Bauer Gerrit E W, Bisogni Valentina

机构信息

National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, NY, USA.

State Key Laboratory of Low Dimensional Quantum Physics, Beijing Tsinghua Institute for Frontier Interdisciplinary Innovation, Beijing, China.

出版信息

Nature. 2025 Sep 10. doi: 10.1038/s41586-025-09488-9.

Abstract

Controlling spin currents, that is, the flow of spin angular momentum, in small magnetic devices, is the principal objective of spin electronics, a main contender for future energy-efficient information technologies. A pure spin current has never been measured directly because the associated electric stray fields and/or shifts in the non-equilibrium spin-dependent distribution functions are too small for conventional experimental detection methods optimized for charge transport. Here we report that resonant inelastic X-ray scattering (RIXS) can bridge this gap by measuring the spin current carried by magnons-the quanta of the spin wave excitations of the magnetic order-in the presence of temperature gradients across a magnetic insulator. This is possible due to the sensitivity of the momentum- and energy-resolved RIXS intensity to minute changes in the magnon distribution under non-equilibrium conditions. We use the Boltzmann equation in the relaxation time approximation to extract transport parameters, such as the magnon lifetime at finite momentum, essential for the realization of magnon spintronics.

摘要

在小型磁性器件中控制自旋电流,即自旋角动量的流动,是自旋电子学的主要目标,自旋电子学是未来节能信息技术的主要竞争者。纯自旋电流从未被直接测量过,因为相关的电杂散场和/或非平衡自旋相关分布函数的变化对于为电荷传输优化的传统实验检测方法来说太小了。在此我们报告,共振非弹性X射线散射(RIXS)可以通过测量在磁绝缘体上存在温度梯度时磁振子(磁有序的自旋波激发量子)所携带的自旋电流来弥合这一差距。这是可行的,因为动量和能量分辨的RIXS强度对非平衡条件下磁振子分布的微小变化很敏感。我们在弛豫时间近似下使用玻尔兹曼方程来提取传输参数,例如有限动量下的磁振子寿命,这对于实现磁振子自旋电子学至关重要。

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