Mietelski J W, Dorda J, Was B
Environmental Radioactivity Lab, Henryk Niewodniczañski Institute of Nuclear Physics, Krakow, Poland.
Appl Radiat Isot. 1999 Oct;51(4):435-47. doi: 10.1016/s0969-8043(99)00055-x.
241Pu activity measurements in coniferous forest soil samples from Poland are presented. The results were obtained in two ways: by alpha spectrometric remeasurements of the plutonium sources 3-4 years after their preparation (i.e. by the 241Am ingrowth) and by direct measurements of 241Pu using liquid scintillation (LS) spectrometry. Both methods gave consistent results. The maximum observed activity concentration obtained by the 241Am ingrowth was (254 +/- 43) Bq/kg, and by direct measurements it was (284 +/- 31) Bq/kg (the same sample, activities calculated for May 1, 1986). Enhanced levels of 241Pu were observed in all samples from the farthest north-eastern Poland. The estimated 241Pu maximum deposition from Chernobyl fallout in this area (sum of deposition for two examined layers of one site) was (1.025 +/- 0.110) kBq/m2. This will result after 70 years in an additional 241Am activity of about (30.1 +/- 3.2) Bq/m2. The average ratio for 241Pu to total 238,239,240Pu was of the order of 25. The obtained average Chernobyl ratios for 241Pu to 239,240Pu were about 86, and those for 241Pu to 238,239,240Pu were 56.
