Thakker D R, Yagi H, Lu A Y, Levin W, Conney A H
Proc Natl Acad Sci U S A. 1976 Oct;73(10):3381-5. doi: 10.1073/pnas.73.10.3381.
Metabolites of (+/-)-trans 7,8-dihydroxy-7,8-dihydrobenzo[a]pyrene formed by a rat liver microsomes and by a highly purified monoxygenase system were analyzed by high-pressure liquid chromatography. Four stereoisomeric tetraols of 7,8,9,10-tetrahydrobenzo[a]pyrene, known solvolysis products of the two highly mutagenic stereoisomers of the 9,10-epoxide of the 7,8-dihydrodiol, were identified as products. The ratio of the two highly unstable diol epoxides formed (7 beta,8alpha-dihydroxy-9beta,10beta-epoxy-7,8,9,10-tetrahydrobenzo[a]pyrene, diol epoxide 1; 7beta,8alpha-dihydroxy-9alpha,10alpha-epoxy-7,8,9,10-tetrahydrobenzo[a]pyrene, diol epoxide 2) ranged from about 1.7 to 0.4. The diol epoxides are sufficiently reactive to alkylate phosphate buffer (pH 7.4) at 37 degrees. Microsomes, particularly those from control animals, formed a substantial amount of an additional metabolite that appears to be phenolic. In analogy to benzo[a]pyrene, the metabolism of the 7,8-dihydrodiol shows similar induction after pretreatment of rats with phenobarbital or 3-methylcholanthrene. Neither diol epoxide appears to be a substrate for epoxide hydrase based on the ratis of tetraols formed in the presence or absence of epoxide hydrase. In view of the known carcinogenicity of benzo[a]pyrene 7,8-oxide and 7,8-dihydrodiol and of the marked mutagenicity of the stereoisomeric diol epoxides, both of these diol epoxides qualify for consideration as "ultimate carcinogen(s)" of benzo[a]pyrene.
通过高压液相色谱法分析了由大鼠肝微粒体和高度纯化的单加氧酶系统形成的(±)-反式7,8-二羟基-7,8-二氢苯并[a]芘的代谢产物。鉴定出了7,8,9,10-四氢苯并[a]芘的四种立体异构四醇,它们是7,8-二氢二醇的9,10-环氧化物的两种高致突变性立体异构体的已知溶剂解产物。所形成的两种高度不稳定的二醇环氧化物(7β,8α-二羟基-9β,10β-环氧-7,8,9,10-四氢苯并[a]芘,二醇环氧化物1;7β,8α-二羟基-9α,10α-环氧-7,8,9,10-四氢苯并[a]芘,二醇环氧化物2)的比例范围约为1.7至0.4。二醇环氧化物具有足够的反应活性,可在37℃下使磷酸盐缓冲液(pH 7.4)烷基化。微粒体,尤其是来自对照动物的微粒体,形成了大量似乎是酚类的额外代谢产物。与苯并[a]芘类似,在用苯巴比妥或3-甲基胆蒽预处理大鼠后,7,8-二氢二醇的代谢表现出相似的诱导作用。基于在存在或不存在环氧化物水合酶的情况下形成的四醇的比例,两种二醇环氧化物似乎都不是环氧化物水合酶的底物。鉴于苯并[a]芘7,8-氧化物和7,8-二氢二醇已知具有致癌性,以及立体异构二醇环氧化物具有明显的致突变性,这两种二醇环氧化物都有资格被视为苯并[a]芘的“最终致癌物”。