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奥地利森林地区臭氧临界水平建模。AOT40概念的修正。

Modelling critical levels of ozone for the forested area of Austria. Modifications of the AOT40 concept.

作者信息

Loibl Wolfgang, Bolhàr-Nordenkampf Harald R, Herman Friedl, Smidt Stefan

机构信息

ARC Systems Research, Austrian Research Centers, A-2444 Seibersdorf, Austria.

出版信息

Environ Sci Pollut Res Int. 2004;11(3):171-80. doi: 10.1007/BF02979672.

Abstract

GOAL, SCOPE AND BACKGROUND: Ozone is the most important air pollutant in Europe for forest ecosystems and the increase in the last decades is significant. The ozone impact on forests can be calculated and mapped based on the provisional European Critical Level (AOT40 = accumulated exposure over a threshold of 40 ppb, 10,000 ppb x h for 6 months of one growing season calculated for 24 h day(-1)). For Norway spruce, the Austrian main tree species, the ozone risk was assessed in a basis approach and because the calculations do not reflect the health status of forests in Austria, the AOT40 concept was developed.

METHODS

Three approaches were outlined and maps were generated for Norway spruce forests covering the entire area of Austria. The 1st approach modifies the AOT40 due to the assumption that forests have adapted to the pre-industrial levels of ozone, which increase with altitude (AOTalt). The 2nd approach modifies the AOT40 according to the ozone concentration in the sub-stomata cavity. This approach is based on such factors as light intensity and water vapour saturation deficit, which affect stomatal uptake (AOTsto). The 3rd approach combines both approaches and includes the hemeroby. The pre-industrial ozone level approach was applied for autochthonous ('natural') forest areas, the ozone-uptake approach for non-autochthonous ('altered') forest areas.

RESULTS AND DISCUSSION

The provisional Critical Level (AOT40) was established to allow a uniform assessment of the ozone risk for forested areas in Europe. In Austria, where ozone risk is assessed with utmost accuracy due to the dense grid of monitoring plots of the Forest Inventory and because the continuously collected data from more than 100 air quality measuring stations, an exceedance up to the five fold of the Critical Level was found. The result could lead to a yield loss of up to 30-40% and to a severe deterioration in the forest health status. However, the data of the Austrian Forest Inventory and the Austrian Forest Damage Monitoring System do not reflect such an ozone impact. Therefore, various approaches were outlined including the tolerance and avoidance mechanisms of Norway spruce against ozone impact. Taking into consideration the adaptation of forests to the pre-industrial background level of ozone, the AOT40 exceedances are markedly reduced (1st approach). Taking into account the stomatal uptake of ozone, unrealistic high amounts of exceedances up to 10,000 ppb x h were found. The modelled risk does not correspond with the health status and the wood increment of the Austrian forests (2nd approach). Consolidating the forgoing two approaches, a final map including the hemeroby was generated. It became clear that the less natural ('altered') forested regions are highly polluted. This means, that more than half of the spruce forests are endangered by ozone impact and AOT40 values of up to 30,000 ppb x h occur (3rd approach).

CONCLUSIONS

The approaches revealed that a plausible result concerning the ozone impact on spruce forests in Austria could only be reached by combining pre-industrial ozone levels, ozone flux into the spruce needles and the hemeroby of forests.

摘要

目标、范围及背景:对于森林生态系统而言,臭氧是欧洲最重要的空气污染物,且在过去几十年中其含量显著增加。基于欧洲临时临界水平(AOT40 = 累积暴露量,超过40 ppb的阈值,一个生长季节6个月内,按每天24小时计算为10,000 ppb·小时),可以计算并绘制臭氧对森林的影响。对于奥地利的主要树种挪威云杉,采用基础方法评估臭氧风险,由于这些计算未反映奥地利森林的健康状况,因此开发了AOT40概念。

方法

概述了三种方法,并为覆盖奥地利全境的挪威云杉林生成了地图。第一种方法修改AOT40,原因是假设森林已适应工业化前的臭氧水平,该水平随海拔升高而增加(AOTalt)。第二种方法根据气孔下腔中的臭氧浓度修改AOT40。此方法基于光照强度和水汽饱和亏缺等影响气孔吸收的因素(AOTsto)。第三种方法结合了前两种方法,并纳入了人为干扰程度。工业化前臭氧水平方法应用于原生(“天然”)林区,臭氧吸收方法应用于非原生(“改变”)林区。

结果与讨论

建立临时临界水平(AOT40)是为了对欧洲林区的臭氧风险进行统一评估。在奥地利,由于森林清查监测地块密集,且有来自100多个空气质量测量站的连续收集数据,因此能够极其准确地评估臭氧风险,结果发现超标量高达临界水平的五倍。这一结果可能导致高达30 - 40%的产量损失以及森林健康状况严重恶化。然而,奥地利森林清查和奥地利森林损害监测系统的数据并未反映出这种臭氧影响。因此,概述了各种方法,包括挪威云杉对臭氧影响的耐受和规避机制。考虑到森林对工业化前臭氧背景水平的适应,AOT40超标量显著降低(第一种方法)。考虑到臭氧的气孔吸收,发现超标量高达10,000 ppb·小时,这一数值过高不符合实际情况。模拟的风险与奥地利森林的健康状况和木材生长量不相符(第二种方法)。综合上述两种方法,生成了一张包含人为干扰程度的最终地图。很明显,自然程度较低(“改变”)的林区污染严重。这意味着,超过一半的云杉林受到臭氧影响的威胁,并且出现了高达30,000 ppb·小时的AOT40值(第三种方法)。

结论

这些方法表明,只有将工业化前的臭氧水平、进入云杉针叶的臭氧通量以及森林的人为干扰程度相结合,才能得出关于臭氧对奥地利云杉林影响的合理结果。

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