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颗粒流体中的笼蔽动力学。

Caging dynamics in a granular fluid.

作者信息

Reis P M, Ingale R A, Shattuck M D

机构信息

Benjamin Levich Institute, The City College of the City University of New York, 140th Street and Convent Avenue, New York, New York 10031, USA.

出版信息

Phys Rev Lett. 2007 May 4;98(18):188301. doi: 10.1103/PhysRevLett.98.188301. Epub 2007 Apr 30.

Abstract

We report an experimental investigation of the caging motion in a uniformly heated granular fluid for a wide range of filling fractions, varphi. At low varphi the classic diffusive behavior of a fluid is observed. However, as varphi is increased, temporary cages develop and particles become increasingly trapped by their neighbors. We statistically analyze particle trajectories and observe a number of robust features typically associated with dense molecular liquids and colloids. Even though our monodisperse and quasi-2D system is known to not exhibit a glass transition, we still observe many of the precursors usually associated with glassy dynamics. We speculate that this is due to a process of structural arrest provided, in our case, by the presence of crystallization.

摘要

我们报告了一项针对均匀加热的颗粒流体在广泛填充率φ范围内的笼形运动的实验研究。在低φ时,观察到流体的经典扩散行为。然而,随着φ的增加,会形成临时笼,粒子越来越多地被其相邻粒子困住。我们对粒子轨迹进行统计分析,并观察到许多通常与稠密分子液体和胶体相关的稳健特征。尽管我们的单分散准二维系统已知不会表现出玻璃化转变,但我们仍然观察到许多通常与玻璃态动力学相关的先兆现象。我们推测这是由于在我们的案例中,由结晶的存在提供的结构停滞过程所致。

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