Reis P M, Ingale R A, Shattuck M D
Benjamin Levich Institute, The City College of the City University of New York, 140th Street and Convent Avenue, New York, New York 10031, USA.
Phys Rev Lett. 2007 May 4;98(18):188301. doi: 10.1103/PhysRevLett.98.188301. Epub 2007 Apr 30.
We report an experimental investigation of the caging motion in a uniformly heated granular fluid for a wide range of filling fractions, varphi. At low varphi the classic diffusive behavior of a fluid is observed. However, as varphi is increased, temporary cages develop and particles become increasingly trapped by their neighbors. We statistically analyze particle trajectories and observe a number of robust features typically associated with dense molecular liquids and colloids. Even though our monodisperse and quasi-2D system is known to not exhibit a glass transition, we still observe many of the precursors usually associated with glassy dynamics. We speculate that this is due to a process of structural arrest provided, in our case, by the presence of crystallization.
我们报告了一项针对均匀加热的颗粒流体在广泛填充率φ范围内的笼形运动的实验研究。在低φ时,观察到流体的经典扩散行为。然而,随着φ的增加,会形成临时笼,粒子越来越多地被其相邻粒子困住。我们对粒子轨迹进行统计分析,并观察到许多通常与稠密分子液体和胶体相关的稳健特征。尽管我们的单分散准二维系统已知不会表现出玻璃化转变,但我们仍然观察到许多通常与玻璃态动力学相关的先兆现象。我们推测这是由于在我们的案例中,由结晶的存在提供的结构停滞过程所致。