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单分子磁体中的贝里相位阻塞

Berry-phase blockade in single-molecule magnets.

作者信息

González Gabriel, Leuenberger Michael N

机构信息

NanoScience Technology Center, University of Central Florida, Orlando, Florida 32826, USA.

出版信息

Phys Rev Lett. 2007 Jun 22;98(25):256804. doi: 10.1103/PhysRevLett.98.256804. Epub 2007 Jun 20.

Abstract

We formulate the problem of electron transport through a single-molecule magnet (SMM) in the Coulomb blockade regime taking into account topological interference effects for the tunneling of the large spin of a SMM. The interference originates from spin Berry phases associated with different tunneling paths. We show that, in the case of incoherent spin states, it is essential to place the SMM between oppositely spin-polarized source and drain leads in order to detect the spin tunneling in the stationary current, which exhibits topological zeros as a function of the transverse magnetic field.

摘要

我们考虑单分子磁体(SMM)大自旋隧穿的拓扑干涉效应,阐述了库仑阻塞 regime 下单分子磁体中电子输运的问题。这种干涉源于与不同隧穿路径相关的自旋贝里相位。我们表明,在非相干自旋态的情况下,为了在静态电流中检测到自旋隧穿,必须将单分子磁体置于自旋极化方向相反的源极和漏极之间,该静态电流作为横向磁场的函数呈现出拓扑零点。

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