Science. 1991 Dec 20;254(5039):1750-5. doi: 10.1126/science.254.5039.1750.
Chemical reactions far from equilibrium on solid surfaces may exhibit typical phenomena of nonlinear dynamics, as exemplified by the catalytic oxidation of carbon monoxide on a platinum(110) single-crystal surface. Depending on the external parameters (temperature and partial pressures of the reactants), the temporal variation of the reaction rate may become oscillatory or even chaotic. In a parallel way, the concentration distributions of the adsorbed species on the surface form spatio-temporal patterns including propagating and standing waves, rotating spirals, as well as irregular and rapidly changing structures denoted "chemical turbulence."
远离平衡态的固 体表面化学反应可能表现出典型的非线性动力学现象，例如一氧化碳在铂（110）单晶表面上的催化氧化。根据外部参数（温度和反应物的分压）的不同，反应速率的时间变化可能呈现出振荡甚至混沌。以类似的方式，吸附物种在表面上的浓度分布形成时空模式，包括传播和驻波、旋转螺旋以及不规则和快速变化的结构，这些结构被称为“化学湍流”。
