Hellborg Ragnar, Skog Göran
Department of Physics, Lund University, Sölvegatan 14, SE-223 62 LUND, Sweden.
Mass Spectrom Rev. 2008 Sep-Oct;27(5):398-427. doi: 10.1002/mas.20172.
In this overview the technique of accelerator mass spectrometry (AMS) and its use are described. AMS is a highly sensitive method of counting atoms. It is used to detect very low concentrations of natural isotopic abundances (typically in the range between 10(-12) and 10(-16)) of both radionuclides and stable nuclides. The main advantages of AMS compared to conventional radiometric methods are the use of smaller samples (mg and even sub-mg size) and shorter measuring times (less than 1 hr). The equipment used for AMS is almost exclusively based on the electrostatic tandem accelerator, although some of the newest systems are based on a slightly different principle. Dedicated accelerators as well as older "nuclear physics machines" can be found in the 80 or so AMS laboratories in existence today. The most widely used isotope studied with AMS is 14C. Besides radiocarbon dating this isotope is used in climate studies, biomedicine applications and many other fields. More than 100,000 14C samples are measured per year. Other isotopes studied include 10Be, 26Al, 36Cl, 41Ca, 59Ni, 129I, U, and Pu. Although these measurements are important, the number of samples of these other isotopes measured each year is estimated to be less than 10% of the number of 14C samples.
在本综述中,描述了加速器质谱法(AMS)的技术及其应用。AMS是一种高度灵敏的原子计数方法。它用于检测放射性核素和稳定核素的极低浓度的天然同位素丰度(通常在10^(-12)至10^(-16)范围内)。与传统辐射测量方法相比,AMS的主要优点是使用更小的样品(毫克甚至亚毫克级)和更短的测量时间(少于1小时)。用于AMS的设备几乎完全基于静电串联加速器,尽管一些最新的系统基于略有不同的原理。在当今存在的约80个AMS实验室中,可以找到专用加速器以及较旧的“核物理机器”。用AMS研究最广泛的同位素是^14C。除了放射性碳测年外,这种同位素还用于气候研究、生物医学应用和许多其他领域。每年测量超过100,000个^14C样品。研究的其他同位素包括^10Be、^26Al、^36Cl、^41Ca、^59Ni、^129I、U和Pu。尽管这些测量很重要,但据估计,每年测量的这些其他同位素的样品数量不到^14C样品数量的10%。