Department of Chemistry, University of Texas at San Antonio, San Antonio, Texas 78249-0698, USA.
Anal Chem. 2010 Feb 15;82(4):1299-304. doi: 10.1021/ac902301b.
The relationship between the state of the surface of carbon nanotubes (CNTs) and their electrochemical activity was investigated using the enzyme cofactor dihydronicotinamide adenine dinucleotide (NADH) as a redox probe. The boiling of CNTs in water, while nondestructive, activated them toward the oxidation of NADH, as indicated by a shift in the anodic peak potential of NADH (E(NADH)) from 0.4 V to 0.0 V. The shift in E(NADH) was due to the redox mediation of NADH oxidation by traces of quinone species that were formed on the surface of treated CNTs. The harsher treatment that was comprised of microwaving CNTs in concentrated nitric acid had a similar effect on the E(NADH), and, additionally, it increased the anodic peak current of NADH. The latter correlated with the formation of defects on the surface of acid-microwaved CNTs, as indicated by their Raman spectra. The increase in current was discussed, considering the role of surface mediators on the buckled graphene sheets of acid-microwaved CNTs. The other carbon allotropes, including the edge-plane pyrolytic graphite, graphite powder, and glassy carbon, did not display a comparable activation toward the oxidation of NADH.
采用酶辅因子二氢烟酰胺腺嘌呤二核苷酸(NADH)作为氧化还原探针,研究了碳纳米管(CNTs)表面状态与其电化学活性之间的关系。CNTs 在水中煮沸虽然不会造成破坏,但会使其对 NADH 的氧化具有活性,这表现为 NADH 的阳极峰电位(E(NADH))从 0.4 V 向 0.0 V 发生偏移。E(NADH)发生偏移是由于处理后的 CNTs 表面形成的痕量醌类物质对 NADH 氧化的氧化还原介导作用。更为剧烈的处理方法是将 CNTs 在浓硝酸中进行微波处理,这对 E(NADH)也有类似的影响,并且还增加了 NADH 的阳极峰电流。后者与酸微波处理的 CNTs 表面缺陷的形成有关,这可以从它们的拉曼光谱中看出。电流的增加与酸微波处理的 CNTs 的褶皱石墨烯片表面上的表面介体的作用有关。其他碳同素异形体,包括边缘平面热解石墨、石墨粉末和玻璃碳,对 NADH 的氧化没有表现出类似的活性。