Department of Condensed Matter Physics, Masaryk University, Kotlárská 2, 61137 Brno, Czech Republic.
Phys Rev Lett. 2010 Jul 9;105(2):027204. doi: 10.1103/PhysRevLett.105.027204.
We derive and study a spin one-half Hamiltonian on a honeycomb lattice describing the exchange interactions between Ir4+ ions in a family of layered iridates A2IrO3 (A=Li,Na). Depending on the microscopic parameters, the Hamiltonian interpolates between the Heisenberg and exactly solvable Kitaev models. Exact diagonalization and a complementary spin-wave analysis reveal the presence of an extended spin-liquid phase near the Kitaev limit and a conventional Néel state close to the Heisenberg limit. The two phases are separated by an unusual stripy antiferromagnetic state, which is the exact ground state of the model at the midpoint between two limits.
我们推导出并研究了一个描述层状铱酸盐 A2IrO3(A=Li,Na)中 Ir4+离子之间交换相互作用的、具有半整数自旋的哈密顿量。根据微观参数的不同,哈密顿量在海森堡模型和可精确求解的 Kitaev 模型之间进行插值。精确对角化和补充的自旋波分析揭示了在 Kitaev 极限附近存在扩展的自旋液体相,以及在海森堡极限附近存在传统的奈尔相。这两个相被一个不寻常的条纹反铁磁相隔开,在两个极限的中点处,该相是模型的精确基态。