Haselwandter Christoph A, Phillips Rob
Department of Applied Physics, California Institute of Technology, Pasadena, California 91125, USA.
Phys Rev E Stat Nonlin Soft Matter Phys. 2011 Jun;83(6 Pt 1):061901. doi: 10.1103/PhysRevE.83.061901. Epub 2011 Jun 1.
In recent experiments [M. Dubois, B. Demé, T. Gulik-Krzywicki, J.-C. Dedieu, C. Vautrin, S. Désert, E. Perez, and T. Zemb, Nature (London) 411, 672 (2001)] the spontaneous formation of hollow bilayer vesicles with polyhedral symmetry has been observed. On the basis of the experimental phenomenology it was suggested [M. Dubois, V. Lizunov, A. Meister, T. Gulik-Krzywicki, J. M. Verbavatz, E. Perez, J. Zimmerberg, and T. Zemb, Proc. Natl. Acad. Sci. USA 101, 15082 (2004)] that the mechanism for the formation of bilayer polyhedra is minimization of elastic bending energy. Motivated by these experiments, we study the elastic bending energy of polyhedral bilayer vesicles. In agreement with experiments, and provided that excess amphiphiles exhibiting spontaneous curvature are present in sufficient quantity, we find that polyhedral bilayer vesicles can indeed be energetically favorable compared to spherical bilayer vesicles. Consistent with experimental observations we also find that the bending energy associated with the vertices of bilayer polyhedra can be locally reduced through the formation of pores. However, the stabilization of polyhedral bilayer vesicles over spherical bilayer vesicles relies crucially on molecular segregation of excess amphiphiles along the ridges rather than the vertices of bilayer polyhedra. Furthermore, our analysis implies that, contrary to what has been suggested on the basis of experiments, the icosahedron does not minimize elastic bending energy among arbitrary polyhedral shapes and sizes. Instead, we find that, for large polyhedron sizes, the snub dodecahedron and the snub cube both have lower total bending energies than the icosahedron.
在最近的实验中[M. 杜波依斯、B. 德梅、T. 古利克 - 克日维茨基、J.-C. 德迪厄、C. 沃特兰、S. 德塞尔、E. 佩雷斯和T. 曾布,《自然》(伦敦)411, 672 (2001)],人们观察到了具有多面体对称性的中空双层囊泡的自发形成。基于实验现象学,有人提出[M. 杜波依斯、V. 利祖诺夫、A. 迈斯特、T. 古利克 - 克日维茨基、J.M. 韦尔巴瓦茨、E. 佩雷斯、J. 齐默伯格和T. 曾布,《美国国家科学院院刊》101, 15082 (2004)],双层多面体形成的机制是弹性弯曲能量的最小化。受这些实验的启发,我们研究了多面体双层囊泡的弹性弯曲能量。与实验一致,并且假设存在足够数量的具有自发曲率的过量两亲分子,我们发现与球形双层囊泡相比,多面体双层囊泡在能量上确实可能更有利。与实验观察结果一致,我们还发现通过形成孔可以局部降低与双层多面体顶点相关的弯曲能量。然而,多面体双层囊泡相对于球形双层囊泡的稳定关键依赖于过量两亲分子沿双层多面体的棱而不是顶点的分子分离。此外,我们的分析表明,与基于实验所提出的情况相反,在任意多面体形状和尺寸中,二十面体并非使弹性弯曲能量最小化。相反,我们发现,对于大尺寸的多面体,截顶十二面体和截顶立方体的总弯曲能量都比二十面体低。