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在电子晶体中快速切换到稳定的隐藏量子态。

Ultrafast switching to a stable hidden quantum state in an electronic crystal.

机构信息

Department of Complex Matter, Jozef Stefan Institute, Jamova 39, Ljubljana SI-1000, Slovenia.

出版信息

Science. 2014 Apr 11;344(6180):177-80. doi: 10.1126/science.1241591.

DOI:10.1126/science.1241591
PMID:24723607
Abstract

Hidden states of matter may be created if a system out of equilibrium follows a trajectory to a state that is inaccessible or does not exist under normal equilibrium conditions. We found such a hidden (H) electronic state in a layered dichalcogenide crystal of 1T-TaS2 (the trigonal phase of tantalum disulfide) reached as a result of a quench caused by a single 35-femtosecond laser pulse. In comparison to other states of the system, the H state exhibits a large drop of electrical resistance, strongly modified single-particle and collective-mode spectra, and a marked change of optical reflectivity. The H state is stable until a laser pulse, electrical current, or thermal erase procedure is applied, causing it to revert to the thermodynamic ground state.

摘要

如果一个处于非平衡状态的系统沿着一条无法达到的轨迹行进,或者在正常平衡条件下不存在,那么物质的隐藏状态就可能被创造出来。我们在 1T-TaS2(二硫化钽的三角相)的层状二卤代物晶体中发现了这样一个隐藏的(H)电子态,这是由于单个 35 飞秒激光脉冲引起的淬火而达到的。与系统的其他状态相比,H 态表现出电阻的大幅下降、强烈修正的单粒子和集体模式谱以及光学反射率的明显变化。H 态是稳定的,直到激光脉冲、电流或热擦除程序被应用,导致它回到热力学基态。

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