Yang Y Y, Liu L Y, Guo L L, Lv Y L, Zhang G M, Lei J, Liu W T, Xiong Y Y, Wen H M
Key Laboratory of Environmental Change and Natural Disaster, Ministry of Education, Beijing Normal University, Beijing, 100875, China,
Environ Monit Assess. 2015 Jul;187(7):409. doi: 10.1007/s10661-015-4611-6. Epub 2015 Jun 7.
The levels and health risks of arsenic and heavy metals (As, Ba, Cd, Co, Cr, Cu, Mn, Ni, Pb, and Zn) in the suspended particulate matter (SPM) collected from an urban household environment in Beijing of China for 12 months were investigated. The mean concentrations of the studied toxic elements were higher and lower than crustal abundance and PM2.5 in the urban outdoors of Beijing. The concentrations of the studied elements displayed significant seasonality. The highest concentrations of the total elements occurred in winter, followed by autumn, while the lowest concentrations were recorded in summer. Based on the calculated values of enrichment factor (EF) and geoaccumulation index (Igeo), the levels for As and Cu were heavily contaminated, while those for Cd, Pb, and Zn were extremely contaminated. As and Pb might pose risks to children and adults via ingestion exposure. The accumulative risks of multi-elements resulted from dermal contact and inhalation exposures were not negligible. More attention should be paid to reducing the non-carcinogenic and carcinogenic health risks posed by the toxic elements bound to urban household SPM particles via ingestion, inhalation, and dermal contact exposure.
对在中国北京城市家庭环境中采集的12个月悬浮颗粒物(SPM)中的砷和重金属(砷、钡、镉、钴、铬、铜、锰、镍、铅和锌)水平及健康风险进行了调查。所研究的有毒元素的平均浓度高于和低于北京城市户外的地壳丰度和PM2.5。所研究元素的浓度呈现出显著的季节性。总元素的最高浓度出现在冬季,其次是秋季,而最低浓度出现在夏季。根据富集因子(EF)和地累积指数(Igeo)的计算值,砷和铜的含量受到严重污染,而镉、铅和锌的含量受到极度污染。砷和铅可能通过摄入暴露对儿童和成人构成风险。皮肤接触和吸入暴露导致的多元素累积风险不可忽视。应更加关注减少通过摄入、吸入和皮肤接触暴露与城市家庭SPM颗粒结合的有毒元素所带来的非致癌和致癌健康风险。