Jacques V L R, Laulhé C, Moisan N, Ravy S, Le Bolloc'h D
Laboratoire de Physique des Solides, CNRS, Univ. Paris-Sud, Université Paris-Saclay, 91405 Orsay Cedex, France.
Synchrotron Soleil, L'Orme des Merisiers, Saint-Aubin, BP 48, 91192 Gif-sur-Yvette Cedex, France.
Phys Rev Lett. 2016 Oct 7;117(15):156401. doi: 10.1103/PhysRevLett.117.156401. Epub 2016 Oct 3.
We report on time-resolved x-ray diffraction measurements following femtosecond laser excitation in pure bulk chromium. Comparing the evolution of incommensurate charge-density-wave (CDW) and atomic lattice reflections, we show that, a few nanoseconds after laser excitation, the CDW undergoes different structural changes than the atomic lattice. We give evidence for a transient CDW shear strain that breaks the lattice point symmetry. This strain is characteristic of sliding CDWs, as observed in other incommensurate CDW systems, suggesting the laser-induced CDW sliding capability in 3D systems. This first evidence opens perspectives for unconventional laser-assisted transport of correlated charges.
我们报道了在纯块状铬中飞秒激光激发后的时间分辨X射线衍射测量结果。通过比较非公度电荷密度波(CDW)和原子晶格反射的演化,我们表明,在激光激发后几纳秒,CDW经历了与原子晶格不同的结构变化。我们提供了瞬态CDW剪切应变破坏晶格点对称性的证据。这种应变是滑动CDW的特征,正如在其他非公度CDW系统中所观察到的,这表明在三维系统中激光诱导的CDW滑动能力。这一初步证据为相关电荷的非常规激光辅助输运开辟了前景。