Gallo-Frantz A, Jacques V L R, Sinchenko A A, Ghoneim D, Ortega L, Godard P, Renault P-O, Hadj-Azzem A, Lorenzo J E, Monceau P, Thiaudière D, Grigoriev P D, Bellec E, Le Bolloc'h D
Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS, 91405, Orsay Cedex, France.
Institut Pprime, CNRS-Université de Poitiers-ENSMA, 86962, Futuroscope-Chasseneuil Cedex, France.
Nat Commun. 2024 Apr 30;15(1):3667. doi: 10.1038/s41467-024-47626-5.
The precise arrangement and nature of atoms drive electronic phase transitions in condensed matter. To explore this tenuous link, we developed a true biaxial mechanical deformation device working at cryogenic temperatures, compatible with x-ray diffraction and transport measurements, well adapted to layered samples. Here we show that a slight deformation of TbTe can have a dramatic influence on its Charge Density Wave (CDW), with an orientational transition from c to a driven by the a/c parameter, a tiny coexistence region near a = c, and without space group change. The CDW transition temperature T displays a linear dependence with while the gap saturates out of the coexistence region. This behaviour is well accounted for within a tight-binding model. Our results question the relationship between gap and T in RTe systems. This method opens a new route towards the study of coexisting or competing electronic orders in condensed matter.
原子的精确排列和性质驱动着凝聚态物质中的电子相变。为了探索这一微弱联系,我们开发了一种在低温下工作的真正双轴机械变形装置,它与X射线衍射和输运测量兼容,非常适合层状样品。在此我们表明,TbTe的轻微变形会对其电荷密度波(CDW)产生显著影响,由a/c参数驱动从c向a发生取向转变,在a = c附近有一个微小的共存区域,且空间群不变。CDW转变温度T与 呈线性依赖关系,而能隙在共存区域之外饱和。这种行为在紧束缚模型中得到了很好的解释。我们的结果对RTe系统中能隙与T之间的关系提出了质疑。该方法为研究凝聚态物质中共存或竞争的电子序开辟了一条新途径。