School of Engineering and Applied Sciences, Harvard University , Pierce Hall, 29 Oxford Street, Cambridge, Massachusetts 02138, United States.
Climate Change Division, Environmental Protection Agency , Washington, District of Columbia 20460, United States.
Environ Sci Technol. 2016 Dec 6;50(23):13123-13133. doi: 10.1021/acs.est.6b02878. Epub 2016 Nov 16.
We present a gridded inventory of US anthropogenic methane emissions with 0.1° × 0.1° spatial resolution, monthly temporal resolution, and detailed scale-dependent error characterization. The inventory is designed to be consistent with the 2016 US Environmental Protection Agency (EPA) Inventory of US Greenhouse Gas Emissions and Sinks (GHGI) for 2012. The EPA inventory is available only as national totals for different source types. We use a wide range of databases at the state, county, local, and point source level to disaggregate the inventory and allocate the spatial and temporal distribution of emissions for individual source types. Results show large differences with the EDGAR v4.2 global gridded inventory commonly used as a priori estimate in inversions of atmospheric methane observations. We derive grid-dependent error statistics for individual source types from comparison with the Environmental Defense Fund (EDF) regional inventory for Northeast Texas. These error statistics are independently verified by comparison with the California Greenhouse Gas Emissions Measurement (CALGEM) grid-resolved emission inventory. Our gridded, time-resolved inventory provides an improved basis for inversion of atmospheric methane observations to estimate US methane emissions and interpret the results in terms of the underlying processes.
我们提供了一个具有 0.1°×0.1°空间分辨率、月度时间分辨率和详细尺度相关误差特征的美国人为甲烷排放网格化清单,与 2016 年美国环境保护署(EPA)的 2012 年美国温室气体排放和汇清单(GHGI)一致。EPA 清单仅作为不同源类型的国家总量提供。我们使用州、县、地方和点源级别的广泛数据库对清单进行细分,并分配各个源类型的排放的空间和时间分布。结果显示与 EDGAR v4.2 全球网格化清单存在很大差异,后者通常作为大气甲烷观测反演的先验估计。我们从与新泽西州东北区环境防御基金(EDF)区域清单的比较中为各个源类型得出了网格相关的误差统计数据。这些误差统计数据通过与加利福尼亚温室气体排放测量(CALGEM)网格分辨排放清单的比较得到独立验证。我们的网格化、时间分辨清单为大气甲烷观测反演提供了改进的基础,以估计美国的甲烷排放,并根据潜在过程解释结果。