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网格化的 2012-2018 年美国人为源甲烷排放清单。

A Gridded Inventory of Annual 2012-2018 U.S. Anthropogenic Methane Emissions.

机构信息

SRON Netherlands Institute for Space Research, Leiden 3584 CA, Netherlands.

Climate Change Division, Environmental Protection Agency, Washington, District of Columbia 20004, United States.

出版信息

Environ Sci Technol. 2023 Oct 31;57(43):16276-16288. doi: 10.1021/acs.est.3c05138. Epub 2023 Oct 19.

DOI:10.1021/acs.est.3c05138
PMID:37857355
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10620993/
Abstract

Nationally reported greenhouse gas inventories are a core component of the Paris Agreement's transparency framework. Comparisons with emission estimates derived from atmospheric observations help identify improvements to reduce uncertainties and increase the confidence in reported values. To facilitate comparisons over the contiguous United States, we present a 0.1° × 0.1° gridded inventory of annual 2012-2018 anthropogenic methane emissions, allocated to 26 individual source categories, with scale-dependent error estimates. Our inventory is consistent with the U.S. Environmental Protection Agency (EPA) Inventory of U.S. Greenhouse Gas Emissions and Sinks (GHGI), submitted to the United Nations in 2020. Total emissions and patterns (spatial/temporal) reflect the activity and emission factor data underlying the GHGI, including many updates relative to a previous gridded version of the GHGI that has been extensively compared with observations. These underlying data are not generally available in global gridded inventories, and comparison to EDGAR version 6 shows large spatial differences, particularly for the oil and gas sectors. We also find strong regional variability across all sources in annual 2012-2018 spatial trends, highlighting the importance of understanding regional- and facility-level activities. Our inventory represents the first time series of gridded GHGI methane emissions and enables robust comparisons of emissions and their trends with atmospheric observations.

摘要

国家报告的温室气体清单是《巴黎协定》透明度框架的核心组成部分。将其与大气观测得出的排放估计值进行比较有助于确定改进措施,以减少不确定性并提高报告值的可信度。为了便于在美国大陆进行比较,我们提供了一份 2012 年至 2018 年人为甲烷排放的 0.1°×0.1°网格化清单,分配给 26 个单独的源类别,并带有与规模相关的误差估计。我们的清单与美国环境保护署(EPA)向联合国提交的 2020 年《美国温室气体排放和汇清单》(GHGI)一致。总排放量和模式(空间/时间)反映了 GHGI 所依据的活动和排放因子数据,包括与之前广泛与观测结果进行比较的 GHGI 网格化版本相比的许多更新。这些基础数据通常在全球网格化清单中不可用,与 EDGAR 版本 6 的比较显示出较大的空间差异,特别是对于石油和天然气部门。我们还发现,在 2012 年至 2018 年的所有来源中,年度空间趋势存在很强的区域变异性,突出了了解区域和设施级活动的重要性。我们的清单代表了 GHGI 甲烷排放的第一个时间序列,并能够对排放及其趋势与大气观测进行稳健比较。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/a51b09c214ef/es3c05138_0005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/a97fd0623bc7/es3c05138_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/e5f9284e86c1/es3c05138_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/919188a351b5/es3c05138_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/9f81a89ac726/es3c05138_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/a51b09c214ef/es3c05138_0005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/a97fd0623bc7/es3c05138_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/e5f9284e86c1/es3c05138_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/919188a351b5/es3c05138_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/9f81a89ac726/es3c05138_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/cd10/10620993/a51b09c214ef/es3c05138_0005.jpg

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