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可见光至近红外光波段下金纳米棒的计算厚度相关等离子体特性。

Calculated thickness dependent plasmonic properties of gold nanobars in the visible to near-infrared light regime.

作者信息

Ghosh Pijush K, Debu Desalegn T, French David A, Herzog Joseph B

机构信息

Department of Physics, University of Arkansas, Fayetteville, Arkansas, United States of America.

Department of Electrical Engineering, University of Arkansas, Fayetteville, Arkansas, United States of America.

出版信息

PLoS One. 2017 May 9;12(5):e0177463. doi: 10.1371/journal.pone.0177463. eCollection 2017.

Abstract

Metallic, especially gold, nanostructures exhibit plasmonic behavior in the visible to near-infrared light range. In this study, we investigate optical enhancement and absorption of gold nanobars with different thicknesses for transverse and longitudinal polarizations using finite element method simulations. This study also reports on the discrepancy in the resonance wavelengths and optical enhancement of the sharp-corner and round-corner nanobars of constant length 100 nm and width 60 nm. The result shows that resonance amplitude and wavelength have strong dependences on the thickness of the nanostructure as well as the sharpness of the corners, which is significant since actual fabricated structure often have rounded corners. Primary resonance mode blue-shifts and broadens as the thickess increases due to decoupling of charge dipoles at the surface for both polarizations. The broadening effect is characterized by measuring the full width at half maximum of the spectra. We also present the surface charge distribution showing dipole mode oscillations at resonance frequency and multimode resonance indicating different oscillation directions of the surface charge based on the polarization direction of the field. Results of this work give insight for precisely tuning nanobar structures for sensing and other enhanced optical applications.

摘要

金属纳米结构,尤其是金纳米结构,在可见光到近红外光范围内表现出等离子体行为。在本研究中,我们使用有限元方法模拟,研究了不同厚度的金纳米棒在横向和纵向偏振下的光学增强和吸收。本研究还报告了长度为100nm、宽度为60nm的等长尖角和圆角纳米棒在共振波长和光学增强方面的差异。结果表明,共振幅度和波长强烈依赖于纳米结构的厚度以及角的尖锐程度,这一点很重要,因为实际制造的结构通常有圆角。由于两种偏振情况下表面电荷偶极子的解耦,随着厚度增加,主要共振模式发生蓝移并展宽。展宽效应通过测量光谱半高全宽来表征。我们还展示了表面电荷分布,显示了共振频率下的偶极子模式振荡以及基于场的偏振方向的多模共振,表明表面电荷的不同振荡方向。这项工作的结果为精确调整纳米棒结构以用于传感和其他增强光学应用提供了见解。

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