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近藤量子自旋液体 α-RuCl 中的中子散射。

Neutron scattering in the proximate quantum spin liquid α-RuCl.

机构信息

Quantum Condensed Matter Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA.

Material Sciences and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA.

出版信息

Science. 2017 Jun 9;356(6342):1055-1059. doi: 10.1126/science.aah6015.

Abstract

The Kitaev quantum spin liquid (KQSL) is an exotic emergent state of matter exhibiting Majorana fermion and gauge flux excitations. The magnetic insulator α-RuCl is thought to realize a proximate KQSL. We used neutron scattering on single crystals of α-RuCl to reconstruct dynamical correlations in energy-momentum space. We discovered highly unusual signals, including a column of scattering over a large energy interval around the Brillouin zone center, which is very stable with temperature. This finding is consistent with scattering from the Majorana excitations of a KQSL. Other, more delicate experimental features can be transparently associated with perturbations to an ideal model. Our results encourage further study of this prototypical material and may open a window into investigating emergent magnetic Majorana fermions in correlated materials.

摘要

Kitaev 量子自旋液体 (KQSL) 是一种奇异的物质涌现状态,表现出马约拉纳费米子和规范通量激发。磁性绝缘体 α-RuCl 被认为实现了近藤 KQSL。我们使用单晶 α-RuCl 上的中子散射来重建能量-动量空间中的动力学相关性。我们发现了非常异常的信号,包括在布里渊区中心附近的大能量间隔上的散射列,其随温度非常稳定。这一发现与 KQSL 的马约拉纳激发的散射一致。其他更微妙的实验特征可以与理想模型的扰动明显相关。我们的结果鼓励对这种原型材料进行进一步研究,并可能为研究关联材料中涌现的磁性马约拉纳费米子开辟一扇窗户。

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