Quantum Condensed Matter Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA.
Material Sciences and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA.
Science. 2017 Jun 9;356(6342):1055-1059. doi: 10.1126/science.aah6015.
The Kitaev quantum spin liquid (KQSL) is an exotic emergent state of matter exhibiting Majorana fermion and gauge flux excitations. The magnetic insulator α-RuCl is thought to realize a proximate KQSL. We used neutron scattering on single crystals of α-RuCl to reconstruct dynamical correlations in energy-momentum space. We discovered highly unusual signals, including a column of scattering over a large energy interval around the Brillouin zone center, which is very stable with temperature. This finding is consistent with scattering from the Majorana excitations of a KQSL. Other, more delicate experimental features can be transparently associated with perturbations to an ideal model. Our results encourage further study of this prototypical material and may open a window into investigating emergent magnetic Majorana fermions in correlated materials.
Kitaev 量子自旋液体 (KQSL) 是一种奇异的物质涌现状态,表现出马约拉纳费米子和规范通量激发。磁性绝缘体 α-RuCl 被认为实现了近藤 KQSL。我们使用单晶 α-RuCl 上的中子散射来重建能量-动量空间中的动力学相关性。我们发现了非常异常的信号,包括在布里渊区中心附近的大能量间隔上的散射列,其随温度非常稳定。这一发现与 KQSL 的马约拉纳激发的散射一致。其他更微妙的实验特征可以与理想模型的扰动明显相关。我们的结果鼓励对这种原型材料进行进一步研究,并可能为研究关联材料中涌现的磁性马约拉纳费米子开辟一扇窗户。