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强约束气溶胶-云相互作用来自火山喷发。

Strong constraints on aerosol-cloud interactions from volcanic eruptions.

机构信息

College of Engineering, Mathematics, and Physical Sciences, University of Exeter, Exeter, UK.

Met Office Hadley Centre, Exeter, UK.

出版信息

Nature. 2017 Jun 22;546(7659):485-491. doi: 10.1038/nature22974.

DOI:10.1038/nature22974
PMID:28640263
Abstract

Aerosols have a potentially large effect on climate, particularly through their interactions with clouds, but the magnitude of this effect is highly uncertain. Large volcanic eruptions produce sulfur dioxide, which in turn produces aerosols; these eruptions thus represent a natural experiment through which to quantify aerosol-cloud interactions. Here we show that the massive 2014-2015 fissure eruption in Holuhraun, Iceland, reduced the size of liquid cloud droplets-consistent with expectations-but had no discernible effect on other cloud properties. The reduction in droplet size led to cloud brightening and global-mean radiative forcing of around -0.2 watts per square metre for September to October 2014. Changes in cloud amount or cloud liquid water path, however, were undetectable, indicating that these indirect effects, and cloud systems in general, are well buffered against aerosol changes. This result will reduce uncertainties in future climate projections, because we are now able to reject results from climate models with an excessive liquid-water-path response.

摘要

气溶胶对气候具有潜在的重大影响,特别是通过它们与云的相互作用,但这种影响的幅度具有高度不确定性。大型火山爆发会产生二氧化硫,进而产生气溶胶;因此,这些爆发代表了一种通过定量气溶胶-云相互作用的自然实验。在这里,我们表明,2014-2015 年冰岛霍拉洪拉火山大规模裂隙喷发减小了液滴云的大小——这与预期一致——但对其他云特性没有明显影响。液滴尺寸的减小导致云变亮,2014 年 9 月至 10 月全球平均辐射强迫约为-0.2 瓦特/平方米。然而,云量或云液水路径的变化无法检测到,这表明这些间接影响,以及一般的云系统,对气溶胶变化有很好的缓冲作用。这一结果将降低未来气候预测的不确定性,因为我们现在能够拒绝对具有过多液水路径响应的气候模型的结果。

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本文引用的文献

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Challenges in constraining anthropogenic aerosol effects on cloud radiative forcing using present-day spatiotemporal variability.利用当前的时空变率来限制人为气溶胶对云辐射强迫的影响所面临的挑战。
Proc Natl Acad Sci U S A. 2016 May 24;113(21):5804-11. doi: 10.1073/pnas.1514036113. Epub 2016 Feb 26.
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Occurrence of pristine aerosol environments on a polluted planet.污染行星上原始气溶胶环境的出现。
Proc Natl Acad Sci U S A. 2014 Dec 30;111(52):18466-71. doi: 10.1073/pnas.1415440111. Epub 2014 Dec 15.
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Large contribution of natural aerosols to uncertainty in indirect forcing.
Sci Rep. 2025 Apr 26;15(1):14653. doi: 10.1038/s41598-025-98811-5.
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High sensitivity of cloud formation to aerosol changes.云形成对气溶胶变化的高敏感性。
Nat Geosci. 2025;18(4):289-295. doi: 10.1038/s41561-025-01662-y. Epub 2025 Apr 3.
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Constraining effects of aerosol-cloud interaction by accounting for coupling between cloud and land surface.通过考虑云与陆地表面之间的耦合来限制气溶胶-云相互作用的影响。
Sci Adv. 2024 May 24;10(21):eadl5044. doi: 10.1126/sciadv.adl5044. Epub 2024 May 23.
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Physical science research needed to evaluate the viability and risks of marine cloud brightening.评估海洋云增亮的可行性和风险所需的物理科学研究。
Sci Adv. 2024 Mar 22;10(12):eadi8594. doi: 10.1126/sciadv.adi8594. Epub 2024 Mar 20.
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Phases in fine volcanic ash.细火山灰中的相。
Sci Rep. 2023 Sep 21;13(1):15728. doi: 10.1038/s41598-023-41412-x.
8
Aerosol effects on clouds are concealed by natural cloud heterogeneity and satellite retrieval errors.气溶胶对云的影响被自然云的不均匀性和卫星反演误差所掩盖。
Nat Commun. 2022 Nov 30;13(1):7357. doi: 10.1038/s41467-022-34948-5.
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Invisible ship tracks show large cloud sensitivity to aerosol.无形的船迹表明云对气溶胶非常敏感。
Nature. 2022 Oct;610(7930):101-106. doi: 10.1038/s41586-022-05122-0. Epub 2022 Oct 5.
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Dual-field-of-view high-spectral-resolution lidar: Simultaneous profiling of aerosol and water cloud to study aerosol-cloud interaction.双视场高光谱分辨率激光雷达:气溶胶和云水同时廓线测量研究气溶胶-云相互作用。
Proc Natl Acad Sci U S A. 2022 Mar 8;119(10):e2110756119. doi: 10.1073/pnas.2110756119. Epub 2022 Mar 2.
自然气溶胶对间接强迫不确定性的巨大贡献。
Nature. 2013 Nov 7;503(7474):67-71. doi: 10.1038/nature12674.
4
Satellite methods underestimate indirect climate forcing by aerosols.卫星方法低估了气溶胶的间接气候强迫。
Proc Natl Acad Sci U S A. 2011 Aug 16;108(33):13404-8. doi: 10.1073/pnas.1018526108. Epub 2011 Aug 1.
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7
The impact of humidity above stratiform clouds on indirect aerosol climate forcing.层状云上方湿度对间接气溶胶气候强迫的影响。
Nature. 2004 Dec 23;432(7020):1014-7. doi: 10.1038/nature03174.