Nadarajah Athavan, Sheldon Matthew T
Opt Express. 2017 May 29;25(11):12753-12764. doi: 10.1364/OE.25.012753.
The inverse Faraday effect (IFE) is an opto-magnetic phenomenon that produces static magnetic fields in a wide range of materials during illumination with circularly polarized light. This study analyzes non-magnetic gold (Au) metal nanostructures, providing insight into plasmonic enhancement of the magnetic and optoelectronic phenomena associated with the IFE. We report a simple numerical approach in combination with full-wave optical simulations (finite-difference time-domain method) for tracking the optically-induced motion of electrons inside plasmonic nanostructures that gives rise to the IFE. In addition to static magnetic fields, a circulating drift current is observed, where the direction of current is the same as the chirality of the circularly polarized light. Our results indicate a significant enhancement of this drift current by ~100 times in Au nanoparticles due to larger optical field gradients in comparison with bulk Au films. We also report on the size, geometry, and spectral dependence of the induced drift currents and static magnetic fields, which we predict can exceed 1×10 T under 10 W m optical intensity for spherical Au nanoparticles. Our results inform the development of new classes of magneto-optic and optoelectronic behavior that can be obtained via direct manipulation of electron dynamics by the optical fields inside metals.
逆法拉第效应(IFE)是一种光磁现象,在圆偏振光照射期间,会在多种材料中产生静磁场。本研究分析了非磁性金(Au)金属纳米结构,深入了解了与逆法拉第效应相关的磁和光电现象的等离子体增强效应。我们报告了一种简单的数值方法,并结合全波光学模拟(有限差分时域法)来追踪等离子体纳米结构内部电子的光致运动,这种运动产生了逆法拉第效应。除了静磁场外,还观察到了循环漂移电流,其电流方向与圆偏振光的手性相同。我们的结果表明,与块状金膜相比,由于更大的光场梯度,金纳米颗粒中的这种漂移电流显著增强了约100倍。我们还报告了感应漂移电流和静磁场的尺寸、几何形状及光谱依赖性,我们预测,对于球形金纳米颗粒,在10 W m 的光强度下,感应漂移电流和静磁场可超过1×10 T。我们的研究结果为新型磁光和光电行为的发展提供了依据,这些行为可通过金属内部光场对电子动力学的直接操纵来实现。