Enhancing Coherent Light-Matter Interactions through Microcavity-Engineered Plasmonic Resonances.

Quantum manipulation is challenging in localized-surface plasmon resonances (LSPRs) due to strong dissipations. To enhance quantum coherence, here we propose to engineer the electromagnetic environment of LSPRs by placing metallic nanoparticles (MNPs) in optical microcavities. An analytical quantum model is first built to describe the LSPR-microcavity interaction, revealing the significantly enhanced coherent radiation and the reduced incoherent dissipation. Furthermore, when a quantum emitter interacts with the LSPRs in the cavity-engineered environment, its quantum yield is enhanced over 40 times and the radiative power over one order of magnitude, compared to those in the vacuum environment. Importantly, the cavity-engineered MNP-emitter system can enter the strong coupling regime of cavity quantum electrodynamics, providing a promising platform for the study of quantum plasmonics, quantum information processing, precise sensing, and spectroscopy.