Yu Xiang-Long, Wu Jiansheng
Department of Physics and Institute for Quantum Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, P. R. China.
Phys Chem Chem Phys. 2018 Jan 24;20(4):2296-2307. doi: 10.1039/c7cp07420d.
Two-dimensional group IVA materials (graphene, silicene, germanene, stanene, and plumbene) are promising candidates for realization of the quantum spin Hall effect and for future device applications. We employ density functional theory, tight-binding models, and a Green's function method to systematically investigate their topological properties. From graphene to plumbene, the strength of spin-orbit coupling and the bulk gap increases with increasing atomic mass, and plumbene, as a normal insulator, is totally different from the other four materials, whose ground states are topological insulators. Through detailed analyses of orbital character weights and the evolution of low-energy states around the Γ point, we explain why plumbene is so different. Our quantum transport calculations also indicate that there exist electronic transport channels along edges within the bulk gap of topological insulators. By investigating the effects of external fields on the electronic structures of silicene, germanene, and stanene, we reveal a rich phase diagram and propose two filters with nearly 100% spin polarization. In addition, we present a theoretical design for a spin twister, based on curved two-dimensional topological insulators.
二维IVA族材料(石墨烯、硅烯、锗烯、锡烯和铅烯)是实现量子自旋霍尔效应及未来器件应用的有前途的候选材料。我们采用密度泛函理论、紧束缚模型和格林函数方法系统地研究它们的拓扑性质。从石墨烯到铅烯,自旋轨道耦合强度和体能隙随原子质量增加而增大,并且铅烯作为一种正常绝缘体,与其他四种基态为拓扑绝缘体的材料完全不同。通过对轨道特征权重以及Γ点附近低能态演化的详细分析,我们解释了铅烯为何如此不同。我们的量子输运计算还表明,在拓扑绝缘体的体能隙内沿边缘存在电子输运通道。通过研究外场对硅烯、锗烯和锡烯电子结构的影响,我们揭示了一个丰富的相图,并提出了两种具有近100%自旋极化率的滤波器。此外,我们基于弯曲的二维拓扑绝缘体提出了一种自旋扭转器的理论设计。