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活性胶体在随机后晶格中的扩散、亚扩散和局域化。

Diffusion, subdiffusion, and localization of active colloids in random post lattices.

机构信息

Univ Lyon, Ens de Lyon, Univ Claude Bernard, CNRS, Laboratoire de Physique, F-69342 Lyon, France.

出版信息

Phys Rev E. 2017 Oct;96(4-1):042611. doi: 10.1103/PhysRevE.96.042611. Epub 2017 Oct 26.

Abstract

Combining experiments and theory, we address the dynamics of self-propelled particles in crowded environments. We first demonstrate that motile colloids cruising at constant speed through random lattices undergo a smooth transition from diffusive to subdiffusive to localized dynamics upon increasing the obstacle density. We then elucidate the nature of these transitions by performing extensive simulations constructed from a detailed analysis of the colloid-obstacle interactions. We evidence that repulsion at a distance and hard-core interactions both contribute to slowing down the long-time diffusion of the colloids. In contrast, the localization transition stems solely from excluded-volume interactions and occurs at the void-percolation threshold. Within this critical scenario, equivalent to that of the random Lorentz gas, genuine asymptotic subdiffusion is found only at the critical density where the motile particles explore a fractal maze.

摘要

我们通过实验和理论相结合的方法研究了在拥挤环境中自主运动粒子的动力学。我们首先证明,在随机格子中以恒定速度巡航的运动胶体在增加障碍物密度时会经历从扩散到亚扩散再到局部动力学的平滑转变。然后,我们通过对胶体-障碍物相互作用的详细分析来进行广泛的模拟,阐明了这些转变的本质。我们证明,远距离排斥和硬心相互作用都有助于减缓胶体的长时间扩散。相比之下,定位转变仅源于排除体积相互作用,并在空穴渗透阈值处发生。在这个临界情景中,与随机洛伦兹气体等效,只有在运动粒子探索分形迷宫的临界密度下才会出现真正的渐近亚扩散。

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