Department of Mechanical Engineering , Hanyang University , 17 Haengdang-Dong , Seongdong-Gu, Seoul 133-791 , South Korea.
Department of Chemistry , Kongju National University , Gongju-si, Chungcheongnam-do 32588 , South Korea.
ACS Appl Mater Interfaces. 2018 Jul 18;10(28):24099-24107. doi: 10.1021/acsami.8b03917. Epub 2018 Jul 5.
In this work, silver nanowires (AgNWs) printed on a polyethylene terephthalate substrate using a bar coater were welded via selective wavelength plasmonic flash light irradiation. To achieve high electrical conductivity and transparent characteristics, the wavelength of the flash white light was selectively chosen and irradiated by using high-pass, low-pass, and band-pass filters. The flash white light irradiation conditions such as on-time, off-time, and number of pulses were also optimized. The wavelength range (400-500 nm) corresponding to the plasmonic wavelength of the AgNW could efficiently weld the AgNW films and enhance its conductivity. To carry out in-depth study of the welding phenomena with respect to wavelength, a multiphysics COMSOL simulation was conducted. The welded AgNW films under selective plasmonic flash light welding conditions showed the lowest sheet resistance (51.275 Ω/sq) and noteworthy transmittance (95.3%). Finally, the AgNW film, which was welded by selective wavelength plasmonic flash light with optical filters, was successfully used to make a large area transparent heat film and dye-sensitized solar cells showing superior performances.
在这项工作中,使用棒涂机在聚对苯二甲酸乙二醇酯基底上打印的银纳米线(AgNWs)通过选择性波长等离子体闪光照射进行焊接。为了实现高导电性和透明特性,通过使用高通、低通和带通滤波器来选择性地选择和照射闪光白光的波长。还优化了闪光白光照射条件,如导通时间、关断时间和脉冲数。与 AgNW 的等离子体波长对应的波长范围(400-500nm)可以有效地焊接 AgNW 薄膜并提高其导电性。为了深入研究与波长相关的焊接现象,进行了多物理场 COMSOL 模拟。在选择性等离子体闪光焊接条件下焊接的 AgNW 薄膜表现出最低的方阻(51.275Ω/sq)和值得注意的透光率(95.3%)。最后,使用带有光学滤波器的选择性波长等离子体闪光成功地焊接了 AgNW 薄膜,用于制造大面积透明热膜和染料敏化太阳能电池,表现出优异的性能。