• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利:CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法,用中文像聊天一样搜索,搜遍4000万医学文献。AI智能推荐,让科研检索更轻松。

立即免费搜索

文件翻译

保留排版,准确专业,支持PDF/Word/PPT等文件格式,支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述,25分钟生成高质量综述,智能提取关键信息,辅助科研写作。

立即免费体验

强光物质耦合 regime 中的二维半导体。

Two-dimensional semiconductors in the regime of strong light-matter coupling.

机构信息

Technische Physik and Wilhelm Conrad Röntgen Research Center for Complex Material Systems, Physikalisches Institut, Universität Würzburg, Am Hubland, 97074, Würzburg, Germany.

Ioffe Institute, St. Petersburg, Russia, 194021.

出版信息

Nat Commun. 2018 Jul 12;9(1):2695. doi: 10.1038/s41467-018-04866-6.

DOI:10.1038/s41467-018-04866-6
PMID:30002368
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC6043564/
Abstract

The optical properties of transition metal dichalcogenide monolayers are widely dominated by excitons, Coulomb-bound electron-hole pairs. These quasi-particles exhibit giant oscillator strength and give rise to narrow-band, well-pronounced optical transitions, which can be brought into resonance with electromagnetic fields in microcavities and plasmonic nanostructures. Due to the atomic thinness and robustness of the monolayers, their integration in van der Waals heterostructures provides unique opportunities for engineering strong light-matter coupling. We review first results in this emerging field and outline future opportunities and challenges.

摘要

过渡金属二卤族化合物单层的光学性质主要由激子(库仑束缚的电子-空穴对)决定。这些准粒子表现出巨大的振子强度,并产生窄带、明显的光学跃迁,可以与微腔和等离子体纳米结构中的电磁场产生共振。由于单层的原子薄度和稳健性,它们在范德华异质结构中的集成为工程强的光物质耦合提供了独特的机会。我们首先回顾这一新兴领域的初步成果,并概述未来的机遇和挑战。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0ec6/6043564/3900c1706c0d/41467_2018_4866_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0ec6/6043564/4be3e04d9620/41467_2018_4866_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0ec6/6043564/19f9570356c4/41467_2018_4866_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0ec6/6043564/3900c1706c0d/41467_2018_4866_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0ec6/6043564/4be3e04d9620/41467_2018_4866_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0ec6/6043564/19f9570356c4/41467_2018_4866_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0ec6/6043564/3900c1706c0d/41467_2018_4866_Fig3_HTML.jpg

相似文献

1
Two-dimensional semiconductors in the regime of strong light-matter coupling.强光物质耦合 regime 中的二维半导体。
Nat Commun. 2018 Jul 12;9(1):2695. doi: 10.1038/s41467-018-04866-6.
2
Demonstration of a polariton step potential by local variation of light-matter coupling in a van-der-Waals heterostructure.通过范德华异质结构中光与物质耦合的局部变化来演示极化激元阶跃势。
Opt Express. 2020 Jun 22;28(13):18649-18657. doi: 10.1364/OE.392821.
3
Metasurface of Strongly Coupled Excitons and Nanoplasmonic Arrays.强耦合激子与纳米等离子体阵列的超表面
Nano Lett. 2024 Aug 21;24(33):10090-10097. doi: 10.1021/acs.nanolett.4c02043. Epub 2024 Aug 6.
4
Strong light-matter coupling in van der Waals materials.范德华材料中的强光-物质耦合
Light Sci Appl. 2024 Aug 21;13(1):203. doi: 10.1038/s41377-024-01523-0.
5
Ultrafast dynamics in van der Waals heterostructures.范德华异质结构中的超快动力学
Nat Nanotechnol. 2018 Nov;13(11):994-1003. doi: 10.1038/s41565-018-0298-5. Epub 2018 Nov 5.
6
Exciton polariton interactions in Van der Waals superlattices at room temperature.室温下范德瓦尔斯超晶格中的激子极化激元相互作用。
Nat Commun. 2023 Mar 17;14(1):1512. doi: 10.1038/s41467-023-36912-3.
7
Interlayer excitons in a bulk van der Waals semiconductor.体相范德华半导体中的层间激子
Nat Commun. 2017 Sep 21;8(1):639. doi: 10.1038/s41467-017-00691-5.
8
Optical absorption of interlayer excitons in transition-metal dichalcogenide heterostructures.过渡金属二卤化物异质结构中层激子的光吸收。
Science. 2022 Apr 22;376(6591):406-410. doi: 10.1126/science.abm8511. Epub 2022 Apr 21.
9
Enhanced light-matter interaction in two-dimensional transition metal dichalcogenides.二维过渡金属二硫属化物中增强的光与物质相互作用。
Rep Prog Phys. 2022 Mar 8;85(4). doi: 10.1088/1361-6633/ac45f9.
10
Cavity-control of interlayer excitons in van der Waals heterostructures.范德华异质结构中层间激子的腔控制
Nat Commun. 2019 Aug 16;10(1):3697. doi: 10.1038/s41467-019-11620-z.

引用本文的文献

1
Roadmap for Photonics with 2D Materials.二维材料光子学路线图
ACS Photonics. 2025 Jul 24;12(8):3961-4095. doi: 10.1021/acsphotonics.5c00353. eCollection 2025 Aug 20.
2
Enhancing interlayer exciton dynamics by coupling with monolithic cavities via the field-induced Stark effect.通过场致斯塔克效应与单片腔耦合增强层间激子动力学。
Nat Nanotechnol. 2025 Jul 17. doi: 10.1038/s41565-025-01969-2.
3
Femtosecond switching of strong light-matter interactions in microcavities with two-dimensional semiconductors.利用二维半导体在微腔中实现强光与物质相互作用的飞秒级开关。

本文引用的文献

1
Observation of bosonic condensation in a hybrid monolayer MoSe-GaAs microcavity.混合单层 MoSe-GaAs 微腔中玻色凝聚的观测。
Nat Commun. 2018 Aug 16;9(1):3286. doi: 10.1038/s41467-018-05532-7.
2
Photonic-crystal exciton-polaritons in monolayer semiconductors.单层半导体中的光子晶体激子极化激元。
Nat Commun. 2018 Feb 19;9(1):713. doi: 10.1038/s41467-018-03188-x.
3
Observation of Tunable Charged Exciton Polaritons in Hybrid Monolayer WS-Plasmonic Nanoantenna System.可调谐带电荷激子极化激元在混合单层 WS-等离子体纳米天线系统中的观察。
Nat Commun. 2025 Jul 14;16(1):6490. doi: 10.1038/s41467-025-61607-2.
4
Tailoring photoluminescence of WS-microcavity coupling devices in broad visible range.在宽可见范围内定制WS微腔耦合器件的光致发光
Nanophotonics. 2023 Jan 24;12(4):753-760. doi: 10.1515/nanoph-2022-0705. eCollection 2023 Feb.
5
Image polaritons in van der Waals crystals.范德华晶体中的图像极化激元。
Nanophotonics. 2022 Jan 4;11(11):2433-2452. doi: 10.1515/nanoph-2021-0693. eCollection 2022 Jun.
6
Strong coupling between WS monolayer excitons and a hybrid plasmon polariton at room temperature.室温下WS单层激子与混合等离激元极化激元之间的强耦合。
Nanophotonics. 2024 Apr 15;13(15):2847-2856. doi: 10.1515/nanoph-2024-0021. eCollection 2024 Jul.
7
Strong exciton-photon coupling in self-hybridized organic-inorganic lead halide perovskite microcavities.自杂化有机-无机铅卤化物钙钛矿微腔中的强激子-光子耦合
Nanophotonics. 2023 Nov 8;12(23):4297-4306. doi: 10.1515/nanoph-2023-0366. eCollection 2023 Nov.
8
Observation of ultra-large Rabi splitting in the plasmon-exciton polaritons at room temperature.室温下等离子体激元 - 激子极化激元中超大拉比分裂的观测。
Nanophotonics. 2023 Jul 10;12(16):3267-3275. doi: 10.1515/nanoph-2023-0162. eCollection 2023 Aug.
9
Metasurface of Strongly Coupled Excitons and Nanoplasmonic Arrays.强耦合激子与纳米等离子体阵列的超表面
Nano Lett. 2024 Aug 21;24(33):10090-10097. doi: 10.1021/acs.nanolett.4c02043. Epub 2024 Aug 6.
10
Tamm-cavity terahertz detector.塔姆腔太赫兹探测器。
Nat Commun. 2024 Jul 2;15(1):5542. doi: 10.1038/s41467-024-49759-z.
Nano Lett. 2018 Mar 14;18(3):1777-1785. doi: 10.1021/acs.nanolett.7b04965. Epub 2018 Feb 6.
4
In-Plane Propagation of Light in Transition Metal Dichalcogenide Monolayers: Optical Selection Rules.过渡金属二硫属化物单层中光的面内传播:光学选择定则
Phys Rev Lett. 2017 Jul 28;119(4):047401. doi: 10.1103/PhysRevLett.119.047401. Epub 2017 Jul 26.
5
Gate-Controlled Spin-Valley Locking of Resident Carriers in WSe_{2} Monolayers.WSe₂ 单层中驻留载流子的门控自旋 - 谷锁定
Phys Rev Lett. 2017 Sep 29;119(13):137401. doi: 10.1103/PhysRevLett.119.137401. Epub 2017 Sep 27.
6
Radiative control of dark excitons at room temperature by nano-optical antenna-tip Purcell effect.室温下通过纳米光天线尖端的 Purcell 效应实现暗激子的辐射控制。
Nat Nanotechnol. 2018 Jan;13(1):59-64. doi: 10.1038/s41565-017-0003-0. Epub 2017 Nov 20.
7
Strong-coupling of WSe in ultra-compact plasmonic nanocavities at room temperature.室温下超紧凑等离子体纳米腔中 WSe 的强耦合。
Nat Commun. 2017 Nov 3;8(1):1296. doi: 10.1038/s41467-017-01398-3.
8
Direct exciton emission from atomically thin transition metal dichalcogenide heterostructures near the lifetime limit.来自接近寿命极限的原子级薄过渡金属二硫属化物异质结构的直接激子发射。
Sci Rep. 2017 Sep 28;7(1):12383. doi: 10.1038/s41598-017-09739-4.
9
Hybrid organic-inorganic polariton laser.混合有机-无机极化激元激光器。
Sci Rep. 2017 Sep 12;7(1):11377. doi: 10.1038/s41598-017-11726-8.
10
Observation of hybrid Tamm-plasmon exciton- polaritons with GaAs quantum wells and a MoSe monolayer.利用砷化镓量子阱和单层硒化钼观测混合态汤氏表面等离子体激元-极化激元
Nat Commun. 2017 Aug 15;8(1):259. doi: 10.1038/s41467-017-00155-w.