ARC Centre of Excellence in Future Low-Energy Electronics Technologies and Nonlinear Physics Centre, Research School of Physics and Engineering, The Australian National University, Canberra, ACT, 2601, Australia.
Institute of Molecular plus, Tianjin University, 300072, Tianjin, China.
Nat Commun. 2018 Aug 9;9(1):2944. doi: 10.1038/s41467-018-05349-4.
A bosonic condensate of exciton polaritons in a semiconductor microcavity is a macroscopic quantum state subject to pumping and decay. The fundamental nature of this driven-dissipative condensate is still under debate. Here, we gain an insight into spontaneous condensation by imaging long-lifetime exciton polaritons in a high-quality inorganic microcavity in a single-shot optical excitation regime, without averaging over multiple condensate realisations. We demonstrate that condensation is strongly influenced by an incoherent reservoir and that the reservoir depletion, the so-called spatial hole burning, is critical for the transition to the ground state. Condensates of photon-like polaritons exhibit strong shot-to-shot fluctuations and density filamentation due to the effective self-focusing associated with the reservoir depletion. In contrast, condensates of exciton-like polaritons display smoother spatial density distributions and are second-order coherent. Our observations show that the single-shot measurements offer a unique opportunity to study fundamental properties of non-equilibrium condensation in the presence of a reservoir.
半导体微腔中的激子极化激元玻色凝聚体是一种受泵浦和衰减影响的宏观量子态。这种驱动耗散凝聚体的基本性质仍存在争议。在这里,我们通过在单次光学激发条件下对高质量无机微腔中的长寿命激子极化激元进行成像,在不平均多个凝聚态实现的情况下,深入了解自发凝聚。我们证明了凝聚强烈受到非相干储层的影响,并且储层耗尽,即所谓的空间孔烧蚀,对于向基态的转变至关重要。由于与储层耗尽相关的有效自聚焦,类光子极化激元的凝聚体会表现出强烈的单次波动和密度细丝化。相比之下,类激子极化激元的凝聚体显示出更平滑的空间密度分布,并且是二阶相干的。我们的观察结果表明,单次测量提供了一个独特的机会,可以在存在储层的情况下研究非平衡凝聚的基本特性。