Duan Sibin, Du Zhe, Fan Hongsheng, Wang Rongming
Beijing Advanced Innovation Center for Materials Genome Engineering, Beijing Key Laboratory for Magneto-Photoelectrical Composite and Interface Science, School of Mathematics and Physics, University of Science and Technology Beijing, Beijing 100083, China.
Department of Physics, Beihang University, Beijing 100191, China.
Nanomaterials (Basel). 2018 Nov 17;8(11):949. doi: 10.3390/nano8110949.
Platinum-based nanomaterials have attracted much interest for their promising potentials in fields of energy-related and environmental catalysis. Designing and controlling the surface/interface structure of platinum-based nanomaterials at the atomic scale and understanding the structure-property relationship have great significance for optimizing the performances in practical catalytic applications. In this review, the strategies to obtain platinum-based catalysts with fantastic activity and great stability by composition regulation, shape control, three-dimension structure construction, and anchoring onto supports, are presented in detail. Moreover, the structure-property relationship of platinum-based nanomaterials are also exhibited, and a brief outlook are given on the challenges and possible solutions in future development of platinum-based nanomaterials towards catalytic reactions.
铂基纳米材料因其在能源相关和环境催化领域的潜在应用前景而备受关注。在原子尺度上设计和控制铂基纳米材料的表面/界面结构,并理解其结构-性能关系,对于优化实际催化应用中的性能具有重要意义。在这篇综述中,详细介绍了通过组成调控、形状控制、三维结构构建以及锚定在载体上等策略来获得具有优异活性和高稳定性的铂基催化剂。此外,还展示了铂基纳米材料的结构-性能关系,并对铂基纳米材料在催化反应未来发展中的挑战及可能的解决方案进行了简要展望。