Shulga Artem G, Kahmann Simon, Dirin Dmitry N, Graf Arko, Zaumseil Jana, Kovalenko Maksym V, Loi Maria A
Zernike Institute for Advanced Materials , University of Groningen , NL-9747AG Groningen , The Netherlands.
Department of Chemistry and Applied Biosciences , ETH Zürich , CH-8093 Zürich , Switzerland.
ACS Nano. 2018 Dec 26;12(12):12805-12813. doi: 10.1021/acsnano.8b07938. Epub 2018 Dec 14.
The application of light-emitting field-effect transistors (LEFET) is an elegant way of combining electrical switching and light emission in a single device architecture instead of two. This allows for a higher degree of miniaturization and integration in future optoelectronic applications. Here, we report on a LEFET based on lead sulfide quantum dots processed from solution. Our device shows state-of-the-art electronic behavior and emits near-infrared photons with a quantum yield exceeding 1% when cooled. We furthermore show how LEFETs can be used to simultaneously characterize the optical and electrical material properties on the same device and use this benefit to investigate the charge transport through the quantum dot film.
发光场效应晶体管(LEFET)的应用是一种将电开关和发光集成于单一器件架构而非两种架构的巧妙方法。这使得未来的光电应用能够实现更高程度的小型化和集成化。在此,我们报道一种基于溶液处理的硫化铅量子点的LEFET。我们的器件展现出了先进的电子性能,并且在冷却时能发射量子产率超过1%的近红外光子。我们还展示了如何利用LEFET在同一器件上同时表征光学和电学材料特性,并利用这一优势研究电荷在量子点薄膜中的传输。